Enhanced interband optical nonlinearities from coupled quantum wells

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Abstract
The recent, rapid advances in nonlinear chipscale nanophotonics in the visible and near-infrared have been largely driven by manipulating the local dielectric environment proximate to decades-old workhorse bulk nonlinear optical materials, rather than increasing the inherent strength of their nonlinear response. While proposed decades ago, we demonstrate the first, to our knowledge, experimental realization of a new class of designer nonlinear materials that leverage the interband optical transition in asymmetric structures to provide strong second-order susceptibility, χ (2) . Using simple AlGaAs/GaAs coupled quantum wells operating in the near-infrared as a prototype, we observed strong second harmonic generation enhancement of 1550–775 nm over bulk controls. Extracted χ (2) values were as high as 2750 pm/V, which is >7× that of bulk GaAs. Furthermore, measured susceptibilities agreed well with quantum mechanical calculations of χ (2) using layer profiles extracted from electron microscopy. Growth interruptions were employed to improve interfacial abruptness in response to electron microscopy characterization, resulting in increased χ (2) toward the simulation predictions for ideal heterointerfaces. More complex layer designs showed predicted χ (2) up to 7 nm/V. Such materials are anticipated to find myriad applications, including entangled photon generation at telecommunications wavelengths for chipscale quantum information processing.
Funding Information
  • Air Force Office of Scientific Research (FA9550-22-1-0307)
  • National Science Foundation (DMREF-1629330)

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