Tunable high-order coherence in the interference of resonance fluorescence and laser light

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Abstract
Resonance fluorescence arises from the coherent interaction of laser light with a two-level system and constitutes a quantum light source exhibiting single-photon emission and antibunching, making it a fundamental building block for future quantum networks. Our recent work [ Nat. Commun. 16 , 6453 ( 2025 ) 10.1038/s41467-025-61884-x ] demonstrates that under continuous-wave excitation and in the absence of pure dephasing, the single-time joint state of resonance fluorescence and the two-level system can be described by a pure entangled state. Here, we analyze the cross-correlation and auto-correlation properties of the quantum optical field generated by the interference of resonance fluorescence with laser light at the resonance excitation frequency. Simulation results indicate that by varying the intensity or phase of the interfering laser light, the higher-order coherence of the post-interference quantum optical field transitions from anti-bunching to super-bunching behavior, consistent with recent theoretical and experimental advances by mean-field engineering. This approach offers a complementary framework to characterize and manipulate the multiphoton quantum optical fields.
Funding Information
  • National Natural Science Foundation of China (12522419)
  • National Natural Science Foundation of China (U25D8016)
  • National Natural Science Foundation of China (12274223)
  • National Natural Science Foundation of China (12494604)
  • National Natural Science Foundation of China (12494600)
  • Natural Science Foundation of Beijing Municipality (IS23011)

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