Strain engineering of van Hove singularity and coupled itinerant ferromagnetism in quasi-2D oxide superlattices

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Abstract
Engineering van Hove singularities (vHss) near the Fermi level, if feasible, offers a powerful route to control exotic quantum phases in electronic and magnetic behaviors. However, conventional approaches rely primarily on chemical and electrical doping and focus mainly on local electrical or optical measurements, limiting their applicability to coupled functionalities. In this study, a vHs-induced insulator-metal transition coupled with a ferromagnetic phase transition was empirically achieved in atomically designed quasi-2D SrRuO3 (SRO) superlattices via epitaxial strain engineering, which has not been observed in conventional 3D SRO systems. Theoretical calculations revealed that epitaxial strain effectively modulates the strength and energy positions of vHs of specific Ru orbitals, driving correlated phase transitions in the electronic and magnetic ground states. X-ray absorption spectroscopy confirmed the anisotropic electronic structure of quasi-2D SRO modulated by epitaxial strain. Magneto-optic Kerr effect and electrical transport measurements demonstrated modulated magnetic and electronic phases. Furthermore, magneto-electrical measurements detected significant anomalous Hall effect signals and ferromagnetic magnetoresistance, indicating the presence of magnetically coupled charge carriers in the 2D metallic regime. This study establishes strain engineering as a promising platform for tuning vHss and resultant itinerant ferromagnetism of low-dimensional correlated quantum systems.
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Funding Information
  • National Research Foundation of Korea (2021R1A2C2011340)
  • National Research Foundation of Korea (RS-2023-00220471)
  • National Research Foundation of Korea (RS-2023-00281671)
  • National Research Foundation of Korea (RS-2022-NR068223)
  • Korea Institute for Advanced Study (CG083502)
  • National Research Foundation of Korea (2021R1C1C1007017)
  • National Research Foundation of Korea (2021R1A4A1031920)
  • National Research Foundation of Korea (RS-2022-NR068223)
  • KISTI Supercomputing Center (KSC-2022- CRE-0465)
  • National Research Council of Science & Technology (GTL24041-000)

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