Competing correlated states and abundant orbital magnetism in twisted monolayer-bilayer graphene

Authors:
  • MHMinhao He
    Minhao He
  • YZYa-Hui Zhang
    Ya-Hui Zhang
  • YLYuhao Li
    Yuhao Li
  • ZFZaiyao Fei
    Zaiyao Fei
  • KWKenji Watanabe
    Kenji Watanabe
  • TTTakashi Taniguchi
    Takashi Taniguchi
  • XXXiaodong Xu
    Xiaodong Xu
  • MYMatthew Yankowitz
    Matthew Yankowitz

Abstract
Flat band moir\'e superlattices have recently emerged as unique platforms for investigating the interplay between strong electronic correlations, nontrivial band topology, and multiple isospin 'flavor' symmetries. Twisted monolayer-bilayer graphene (tMBG) is an especially rich system owing to its low crystal symmetry and the tunability of its bandwidth and topology with an external electric field. Here, we find that orbital magnetism is abundant within the correlated phase diagram of tMBG, giving rise to the anomalous Hall effect (AHE) in correlated metallic states nearby most odd integer fillings of the flat conduction band, as well as correlated Chern insulator states stabilized in an external magnetic field. The behavior of the states at zero field appears to be inconsistent with simple spin and valley polarization for the specific range of twist angles we investigate, and instead may plausibly result from an intervalley coherent (IVC) state with an order parameter that breaks time reversal symmetry. The application of a magnetic field further tunes the competition between correlated states, in some cases driving first-order topological phase transitions. Our results underscore the rich interplay between closely competing correlated ground states in tMBG, with possible implications for probing exotic IVC ordering.
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