X-ray absorption spectroscopy and x-ray magnetic circular dichroism of epitaxially grown Heusler alloy Co2MnSi ultrathin films facing a MgO barrier

We element specifically studied the electronic and magnetic states of epitaxially grown full-Heusler alloy ${\mathrm{Co}}_2\mathrm{Mn}\mathrm{Si}$ (CMS) $1.1\mathrm{nm}$ (4 ML) thick ultrathin films facing an epitaxial MgO(001) tunnel barrier by means of x-ray absorption spectroscopy (XAS) and x-ray magnetic circular dichroism (XMCD). In situ reflection high-energy electron-diffraction observations indicated that the CMS films grew into the $L{2}_1$ structure. The observed XAS and XMCD spectra revealed that the CMS ultrathin film was not oxidized. The ratio of Mn and Co spin magnetic moments obtained by applying the sum rules was about 2.7, close to a theoretical value of 2.8 for CMS with the $L{2}_1$ structure.