Dephasing of ultracold cesium 80D5/2-Rydberg electromagnetically induced transparency

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Abstract
We study Rydberg electromagnetically induced transparency (EIT) of a cascade three-level atom involving 80D5/2 state in a strong interaction regime employing a cesium ultracold cloud. In our experiment, a strong coupling laser couples 6P3/2 to 80D5/2 transition, while a weak probe, driving 6S1/2 to 6P3/2 transition, probes the coupling induced EIT signal. At the two-photon resonance, we observe that the EIT transmission decreases slowly with time, which is a signature of interaction induced metastability. The dephasing rate γOD is extracted with optical depth OD = γODt. We find that the optical depth linearly increases with time at onset for a fixed probe incident photon number Rin before saturation. The dephasing rate shows a nonlinear dependence on Rin. The dephasing mechanism is mainly attributed to the strong dipole-dipole interactions, which leads to state transfer from nD5/2 to other Rydberg states. We demonstrate that the typical transfer time τ0(80D) obtained by the state selective field ionization technique is comparable with the decay time of EIT transmission τ0(EIT). The presented experiment provides a useful tool for investigating the strong nonlinear optical effects and metastable state in Rydberg many-body systems.
Funding Information
  • Engineering and Physical Sciences Research Council (EP/W015641/1)
  • Shanghai Pujiang Program (21PJ1402500)
  • 1331 Project of Shanxi Province (202104041101015)
  • Changjiang Scholars and Innovative Research Team in University of Ministry of Education of China (RTIRT 17R70)
  • National Natural Science Foundation of China (11904104, 12104337, 12120101004, 12241408, 12274131, 61835007, 62175136)

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