Thermal Light Emission from Monolayer MoS2
- 19 June 2017
- journal article
- research article
- Published by Wiley in Advanced Materials
- Vol. 29 (31)
Abstract
Layered transition metal dichalcogenide semiconductors, such as MoS2 and WSe2, exhibit a range of fascinating properties and are being currently explored for a variety of electronic and optoelectronic devices. These properties include a low thermal conductivity and a large Seebeck coefficient, which make them promising for thermoelectric applications. Moreover, transition metal dichalcogenides undergo an indirect‐to‐direct bandgap transition when thinned down in thickness, leading to strong excitonic photo‐ and electroluminescence in monolayers. Here, it is demonstrated that a MoS2 monolayer sheet, freely suspended in vacuum over a distance of 150 nm, emits visible light as a result of Joule heating. Due to the poor transfer of heat to the contact electrodes, as well as the suppressed heat dissipation through the underlying substrate, the electron temperature can reach ≈1500–1600 K. The resulting narrow‐band light emission from thermally populated exciton states is spatially located to an only ≈50 nm wide region in the center of the device and goes along with a negative differential electrical conductance of the channel.Keywords
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Funding Information
- H2020 Future and Emerging Technologies (696656)
- Austrian Science Fund (Y 539‐N16)
This publication has 56 references indexed in Scilit:
- Mobility engineering and a metal–insulator transition in monolayer MoS2Nature Materials, 2013
- Photoluminescence emission and Raman response of monolayer MoS_2, MoSe_2, and WSe_2Optics Express, 2013
- Carbon-nanotube photonics and optoelectronicsNature Photonics, 2008
- Superior Thermal Conductivity of Single-Layer GrapheneNano Letters, 2008
- Electrically driven thermal light emission from individual single-walled carbon nanotubesNature Nanotechnology, 2007
- Thermally and Molecularly Stimulated Relaxation of Hot Phonons in Suspended Carbon NanotubesThe Journal of Physical Chemistry B, 2006
- Negative Differential Conductance and Hot Phonons in Suspended Nanotube Molecular WiresPhysical Review Letters, 2005
- Energy-Conservation Considerations in the Characterization of Impact Ionization in SemiconductorsPhysical Review B, 1972
- Temperature dependence of the energy gap in semiconductorsPhysica, 1967
- Melting Point and Sublimation of Molybdenum DisulphideNature, 1959