Pressure and Field Induced Magnetic Order in the Spin LiquidTb2Ti2O7as Studied by Single Crystal Neutron Diffraction

We have studied the spin liquid ${\mathrm{T}\mathrm{b}}_2{\mathrm{T}\mathrm{i}}_2{\mathrm{O}}_7$ by single crystal neutron diffraction under high pressure up to 2.8 GPa, together with uniaxial stress, down to 0.1 K, in zero and high magnetic fields up to 7 T. In zero magnetic field, a long-range ordered antiferromagnetic structure is induced by pressure. The Néel temperature and ordered magnetic moment can be tuned by the anisotropic pressure component. Under magnetic field, the antiferromagnetic structure transforms into a canted ferromagnetic one at 0.6 T. Spin canting persists even at 7 T. The magnetic phase diagram under pressure shows a strong increase of the Néel temperature with the field.