Dynamic Nonlinear Behavior of Ionic Liquid-Based Reservoir Computing Devices
Open Access
- 26 July 2022
- journal article
- research article
- Published by American Chemical Society (ACS) in ACS Applied Materials & Interfaces
- Vol. 14 (32) , 36890-36901
Abstract
Herein, a physical reservoir device that uses faradaic currents generated by redox reactions of metal ions in ionic liquids was developed. Synthetic time-series data consisting of randomly arranged binary number sequences ("1" and "0") were applied as isosceles-triangular voltage pulses with positive and negative voltage heights, respectively, and the effects of the faradaic current on short-term memory and parity-check task accuracies were verified. The current signal for the first half of the triangular voltage-pulse period, which contained a much higher faradaic current component compared to that of the second half of the triangular voltage-pulse period, enabled higher short-term memory task accuracy. Furthermore, when parity-check tasks were performed using a faradaic current generated by asymmetric triangular voltage-pulse levels of 1 and 0, the parity-check task accuracy was approximately eight times higher than that of the symmetric triangular voltage pulse in terms of the correlation coefficient between the output signal and target data. These results demonstrate the advantage of the faradaic current on both the short-term memory characteristics and nonlinear conversion capabilities and are expected to provide guidance for designing and controlling various physical reservoir devices that utilize electrochemical reactions.Keywords
Funding Information
- Japan Science and Technology Agency (JPMXPF21NM0006)
This publication has 32 references indexed in Scilit:
- A Reversible and Higher-Rate Li-O 2 BatteryScience, 2012
- Information processing using a single dynamical node as complex systemNature Communications, 2011
- Redox‐Based Resistive Switching Memories – Nanoionic Mechanisms, Prospects, and ChallengesAdvanced Materials, 2009
- Study of the electrochemical deposition of Sn–Ag–Cu alloy by cyclic voltammetry and chronoamperometryElectrochimica Acta, 2009
- Real-Time Computation at the Edge of Chaos in Recurrent Neural NetworksNeural Computation, 2004
- Harnessing Nonlinearity: Predicting Chaotic Systems and Saving Energy in Wireless CommunicationScience, 2004
- Real-Time Computing Without Stable States: A New Framework for Neural Computation Based on PerturbationsNeural Computation, 2002
- Cyclic voltammetry and bioassay of some superoxide dismutase mimetic copper complex compoundsBioelectrochemistry and Bioenergetics, 1997
- Periodic Variations of Overvoltages for Water Electrolysis in Acid Solutions from Cyclic Voltammetric StudiesJournal of the Electrochemical Society, 1976
- A Stochastic Approximation MethodThe Annals of Mathematical Statistics, 1951