Single-Shot Magnetization Reversal in Ferromagnetic Spin Valves via Heat Control
- 9 September 2025
- journal article
- Published by American Physical Society (APS) in Physical Review Letters
- Vol. 135 (11) , 116702
Abstract
We study laser-induced ultrafast magnetization reversal in a ferromagnetic spin valve by comparing the effects of direct laser excitation and ultrashort hot-electron pulses. A wedged Cu layer is deposited atop the spin valve to tune energy transmission to the magnetic stack for both optical and hot-electron excitation. We demonstrate single-shot magnetization reversal of the free layer using hot-electron pulses. Moreover, such reversal is achieved even with picosecond laser pulses. The influence of laser fluence, Cu thickness (t_{Cu}), and pulse duration is investigated in detail. Our results indicate that the key factor enabling magnetization reversal is full demagnetization of the free layer, driven by a rapid rise in its electronic temperature-achieved via either direct laser or hot-electron excitation. This work advances the understanding of ultrafast magnetization reversal via nonlocal heat and spin transport under strongly out-of-equilibrium conditions.Keywords
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Funding Information
- Agence Nationale de la Recherche (ANR-22-PEEL-0009, ANR- 20-CE24- 0003, SLAM ANR- 23-CE30-0047, ANR-15- IDEX-04-LUE)
- European Commission (22J22178)
- Research Council of Finland (316857)
- Sakura Science Exchange Program
- Japan Society for the Promotion of Science (24K22964)
- Tohoku University
- European Cooperation in Science and Technology (CA23136 CHIROMAG)
- Japan Science and Technology Agency (JPMJAP2409)
- Institute Carnot ICEEL
- région grand est
- Metropole Grand Nancy
- Grant-in-Aid for Transformative Research Areas (24H02235)
This publication has 34 references indexed in Scilit:
- Concepts and use cases for picosecond ultrasonics with x-raysPhotoacoustics, 2023
- Atomic Scale Control of Spin Current Transmission at InterfacesNano Letters, 2022
- Engineering Single-Shot All-Optical Switching of Ferromagnetic MaterialsNano Letters, 2020
- Energy Efficient Control of Ultrafast Spin Current to Induce Single Femtosecond Pulse Switching of a FerromagnetAdvanced Science, 2020
- Heat Transport without Heating?—An Ultrafast X‐Ray Perspective into a Metal HeterostructureAdvanced Functional Materials, 2020
- Single‐Shot Multi‐Level All‐Optical Magnetization Switching Mediated by Spin TransportAdvanced Materials, 2018
- Ultrafast Magnetization Manipulation Using Single Femtosecond Light and Hot‐Electron PulsesAdvanced Materials, 2017
- Hot electron lifetimes in metals probed by time-resolved two-photon photoemissionProgress in Surface Science, 2015
- Electron and lattice dynamics following optical excitation of metalsChemical Physics, 2000
- Current-driven excitation of magnetic multilayersJournal of Magnetism and Magnetic Materials, 1996