Visible Light‐Driven Biginelli Reaction over Mesoporous g‐C 3 N 4 Lewis‐Base Catalyst
- 17 April 2018
- journal article
- research article
- Published by Wiley in ChemistrySelect
- Vol. 3 (14) , 4009-4014
Abstract
In current work, we explore a new catalytic approach to multicomponent Biginelli condensation using mesoporous graphitic carbon nitride (mpg‐C 3 N 4 ) as heterogeneous Lewis‐base catalyst. Present protocol provides solvent free, mild reaction condition, optimal yield and easy separation of catalyst. This method also offers ample yield of pure products within very short reaction time. Heterogeneously dispersed mpg‐C 3 N 4 catalyst is stable and recyclable with consistent catalytic activity under visible light irradiation.Keywords
Funding Information
- Akanksha Gupta
This publication has 33 references indexed in Scilit:
- Synthesis of Ag/g‐C3N4 Composite as Highly Efficient Visible‐Light Photocatalyst for Oxidative Amidation of Aromatic AldehydesAdvanced Synthesis & Catalysis, 2016
- Nanospherical Carbon Nitride Frameworks with Sharp Edges Accelerating Charge Collection and Separation at a Soft Photocatalytic InterfaceAdvanced Materials, 2014
- Iodine Modified Carbon Nitride Semiconductors as Visible Light Photocatalysts for Hydrogen EvolutionAdvanced Materials, 2013
- A Facile Band Alignment of Polymeric Carbon Nitride Semiconductors to Construct Isotype HeterojunctionsAngewandte Chemie International Edition, 2012
- Polymeric Graphitic Carbon Nitride as a Heterogeneous Organocatalyst: From Photochemistry to Multipurpose Catalysis to Sustainable ChemistryAngewandte Chemie International Edition, 2011
- Visible‐Light‐Induced Metal‐Free Allylic Oxidation Utilizing a Coupled Photocatalytic System of g‐C3N4 and N‐Hydroxy CompoundsAdvanced Synthesis & Catalysis, 2011
- Nitrogen‐Doped Carbon Materials Prepared by Ammoxidation as Solid Base Catalysts for Knoevenagel Condensation and Transesterification ReactionsAdvanced Synthesis & Catalysis, 2010
- Two‐Dimensional Hexagonally‐Ordered Mesoporous Carbon Nitrides with Tunable Pore Diameter, Surface Area and Nitrogen ContentAdvanced Functional Materials, 2008
- Chemical Synthesis of Mesoporous Carbon Nitrides Using Hard Templates and Their Use as a Metal‐Free Catalyst for Friedel–Crafts Reaction of BenzeneAngewandte Chemie International Edition, 2006
- Preparation and Characterization of Well‐Ordered Hexagonal Mesoporous Carbon NitrideAdvanced Materials, 2005