Layered Thiazolo[5,4-d] Thiazole-Linked Conjugated Microporous Polymers with Heteroatom Adoption for Efficient Photocatalysis Application

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Abstract
Conjugated microporous polymers (CMPs) with high surface areas, tunable building blocks and fully conjugated structures have found important applications in optoelectronic. Here we report a new series of CMPs with tunable band gaps by introducing thiazolo[5,4-d] thiazole as the linkage. Because they are synthetic polymers, the geometries and structures could be rationally designed. Their intrinsic wide visible light absorption properties and layered architectures endow them with promising photocatalysis performance. The role of the geometries, surface areas and morphologies of the CMPs on the photocatalysis abilities are examined and discussed. The results indicate that geometries have a direct impact on the surface areas and morphologies of the CMPs and thus exert great influence on the photocatalysis
Funding Information
  • National Natural Science Foundation of China (21604028, 21875078)
  • Huazhong University of Science and Technology (2016JCTD104)
  • China Postdoctoral Science Foundation (2017M622423)
  • Ministry of Science and Technology of the People's Republic of China (2016YFE0124400)

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