Magnetic behavior of Ce(Cu1−xAgx)6

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Abstract
We have investigated doped CeCu6 via x-ray diffraction, dc and ac susceptibility, and specific heat in zero and applied magnetic field with a primary focus on the magnetic behavior caused by Ag doping. We present evidence from bulk specific heat and metallography data that the limit of Ag solubility in Ce(Cu1−x Agx )6 is x∼0.1. Data below the magnetic ordering temperature may be fit to an exponential temperature dependence, implying a weak-coupled energy gap of Δ=0.58 K, contradicting an earlier report that C behaves linearly with temperature with a γ over 3 J/mol K2 in the ordered state. Comparisons to magnetically ordered, doped UPt3 are made.

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