Recombination dynamics of localized excitons in cubic InxGa1−xN/GaN multiple quantum wells grown by radio frequency molecular beam epitaxy on 3C–SiC substrate
- 1 July 2003
- journal article
- Published by American Vacuum Society in Journal of Vacuum Science & Technology B: Microelectronics and Nanometer Structures Processing, Measurement, and Phenomena
- Vol. 21 (4) , 1856-1862
Abstract
Recombination dynamics of localized excitons in strained cubic multiple quantum wells (MQWs) grown on 3C–SiC (001) were summarized in terms of well thickness L, InN molar fraction x, and temperature T. Photoluminescence (PL) peak energy of MQWs showed a moderate blueshift as L decreased, and the low-temperature PL lifetime did not change remarkably by changing L. These results proved that the quantum-confined Stark effect due either to spontaneous or piezoelectric polarization was inactive in cubic polytypes. Consequently, time-resolved PL (TRPL) data of MQWs reflect the intrinsic exciton dynamics. The TRPL signal showed stretched exponential decay and spectral redshift with time after excitation up to 300 K. The results are fingerprints that the spontaneous emission is due to the radiative recombination of excitons localized in disordered quantum nanostructures forming extended and localized states. Effective localization depth increased with the increase in x, which gave rise to fast exciton localization. However, nonradiative lifetime in the free or extended states decreased more rapidly with the increase in x and T, giving the emission efficiency maximum at particular x around 0.1.
Keywords
This publication has 43 references indexed in Scilit:
- Structural and optical properties of InAlGaN films grown directly on low-temperature buffer layer with (0001) sapphire substrateJournal of Crystal Growth, 2003
- Localized exciton dynamics in strained cubic In0.1Ga0.9N/GaN multiple quantum wellsApplied Physics Letters, 2001
- Self-trapped exciton recombination in silicon nanocrystalsPhysical Review B, 2001
- The origin of optical gain in cubic InGaN grown by molecular beam epitaxyApplied Physics Letters, 2000
- Exciton Spectra of Cubic and Hexagonal GaN Epitaxial FilmsJapanese Journal of Applied Physics, 1997
- Recombination dynamics of localized excitons in N-N multiple quantum wellsPhysical Review B, 1997
- Stretched-exponential decay of the luminescence in porous siliconPhysical Review B, 1993
- GaN, AlN, and InN: A reviewJournal of Vacuum Science & Technology B: Microelectronics and Nanometer Structures Processing, Measurement, and Phenomena, 1992
- Exciton Transfer between Localized States in CdS1–xSex AlloysPhysica Status Solidi (b), 1989
- Cubic phase gallium nitride by chemical vapour depositionPhysica Status Solidi (a), 1974