Shaping the Infrared luminescence of Colloidal Nanocrystals Using a Dielectric Microcavity

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Abstract
As they have gained maturity, colloidal nanocrystals (NCs) have also expand the spectral range over of which they could be used for photonic and optoelectronic applications. In particular, the infrared use of NCs has become of utmost interest to develop cost‐effective alternatives to current technologies. It is then critical not to let the material dictate the light–matter interaction, which is why the coupling of NCs to photonic cavities has been proposed. For infrared NCs, this approach has first been devoted to the control of absorption with in mind the increase of the signal magnitude for detectors. A Lot of efforts have been focused on the use of metallic metasurfaces. However, these generate significant optical losses and yield low quality factor. Here, this study rather focus on the coupling of infrared NCs to a dielectric mirror cavity. HgTe/CdS core‐shell NCs are used and integrated into a cavity made of aperiodic dielectric mirrors. The effect of the substrate is systematically study on spectral linewidth, carrier dynamic, and emission directivity. The cavity is shown to narrow the PL by a factor 10, while focusing the emission over a 12° angle. Monitoring the power dependence of the emission, this study shows that the cavity leads to 250 K increase in the effective electronic temperature.
Funding Information
  • H2020 European Research Council (AQDtive(n°101086358), Forward(n°771688))
  • Agence Nationale de la Recherche (E‐map(ANR‐22‐CE50‐0025), Bright(ANR‐21‐CE24‐0012), MixDFerro(ANR‐21‐CE09‐0029), Quicktera(ANR‐22‐CE09‐0018), Operatwist(ANR‐22‐CE09‐0037), ANR‐10‐LABX‐0035), Graskop(ANR‐19‐CE09‐0026), Frontal(ANR‐19‐CE24‐0022))
  • U.S. Department of Energy (DE‐AC02‐06CH11357)
  • European Research Council (Ne2dem(grantn°853049))

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