Inhomogeneous Mode-Coupling Theory and Growing Dynamic Length in Supercooled Liquids
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- 6 November 2006
- journal article
- research article
- Published by American Physical Society (APS) in Physical Review Letters
- Vol. 97 (19) , 195701
Abstract
We extend mode-coupling theory (MCT) to inhomogeneous situations, relevant for supercooled liquid in an external field. We compute the response of the dynamical structure factor to a static inhomogeneous external potential and provide the first direct evidence that the standard formulation of MCT is associated with a diverging length scale. We find that the so-called cages are, in fact, extended objects. Although close to the transition the dynamic length grows as in both the and regimes, our results suggest that the fractal dimension of correlated clusters is larger in the regime. We derive inhomogeneous MCT equations valid to second order in gradients.
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