Inhomogeneous Mode-Coupling Theory and Growing Dynamic Length in Supercooled Liquids

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Abstract
We extend mode-coupling theory (MCT) to inhomogeneous situations, relevant for supercooled liquid in an external field. We compute the response of the dynamical structure factor to a static inhomogeneous external potential and provide the first direct evidence that the standard formulation of MCT is associated with a diverging length scale. We find that the so-called cages are, in fact, extended objects. Although close to the transition the dynamic length grows as |T−Tc|−1/4 in both the β and α regimes, our results suggest that the fractal dimension of correlated clusters is larger in the α regime. We derive inhomogeneous MCT equations valid to second order in gradients.
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