A self‐adaptive, data‐driven method to predict the cycling life of lithium‐ion batteries
Authors:
Open Access
Abstract
Accurately forecasting the nonlinear degradation of lithium‐ion batteries (LIBs) using early‐cycle data can obviously shorten the battery test time, which accelerates battery optimization and production. In this work, a self‐adaptive long short‐term memory (SA‐LSTM) method has been proposed to predict the battery degradation trajectory and battery lifespan with only early cycling data. Specifically, two features were extracted from discharge voltage curves by a time‐series‐based approach and forecasted to further cycles using SA‐LSTM model. The as‐obtained features were correlated with the capacity to predict the capacity degradation trajectory by generalized multiple linear regression model. The proposed method achieved an average online prediction error of 6.00% and 6.74% for discharge capacity and end of life, respectively, when using the early‐cycle discharge information until 90% capacity retention. Furthermore, the importance of temperature control was highlighted by correlating the features with the average temperature in each cycle. This work develops a self‐adaptive data‐driven method to accurately predict the cycling life of LIBs, and unveils the underlying degradation mechanism and the importance of controlling environmental temperature. imageKeywords
Funding Information
- National Key Research and Development Program of China (2021YFB2500300)
- Natural Science Foundation of Beijing Municipality (Z200011)
- National Natural Science Foundation of China (21825501, 22379121, 22209094, 22209093, T2322015)
- Fundamental Research Funds for the Central Universities
This publication has 54 references indexed in Scilit:
- Gaussian process regression for forecasting battery state of healthJournal of Power Sources, 2017
- On the Suitability of Electrochemical-Based Modeling for Lithium-Ion BatteriesIEEE Transactions on Transportation Electrification, 2016
- Application of machine learning methods for the prediction of crystal system of cathode materials in lithium-ion batteriesComputational Materials Science, 2016
- Theory of SEI Formation in Rechargeable Batteries: Capacity Fade, Accelerated Aging and Lifetime PredictionJournal of the Electrochemical Society, 2012
- Prognostics of lithium-ion batteries based on Dempster–Shafer theory and the Bayesian Monte Carlo methodJournal of Power Sources, 2011
- A Mathematical Model for the Lithium-Ion Negative Electrode Solid Electrolyte InterphaseJournal of the Electrochemical Society, 2004
- An accelerated calendar and cycle life study of Li-ion cellsJournal of Power Sources, 2001
- Mathematical Modeling of the Lithium Deposition Overcharge Reaction in Lithium‐Ion Batteries Using Carbon‐Based Negative ElectrodesJournal of the Electrochemical Society, 1999
- Determination of state-of-charge and state-of-health of batteries by fuzzy logic methodologyJournal of Power Sources, 1999
- Modeling of Galvanostatic Charge and Discharge of the Lithium/Polymer/Insertion CellJournal of the Electrochemical Society, 1993