Composition and magnetic character of nanometre-size Cu precipitates in reactor pressure vessel steels: Implications for nuclear power plant lifetime extension
Authors:
- P. Asoka-KumarPAP. Asoka-Kumar
- B.D. WirthBWB.D. Wirth
- P.A. SternePSP.A. Sterne
- R.H. HowellRHR.H. Howell
- G.R. OdetteGOG.R. Odette
- 14 November 2002
- journal article
- research article
- Published by Taylor & Francis in Philosophical Magazine Letters
- Vol. 82 (11) , 609-615
Abstract
The sensitivity of positrons to nanometre-size Cu precipitates in Fe alloys has enabled us to apply a novel spin-polarized element-specific method to probe the composition and magnetic character of the precipitates responsible for reactor pressure vessel (RPV) steel embrittlement. The results clearly show that the precipitates are non-magnetic and place an upper limit of about 10at% on their Fe content. The practical implication of this result is that the Cu precipitate contribution to RPV steel embrittlement saturates is not expected to contribute further during lifetime extension. Our study demonstrates that polarized positrons can be used as a powerful probe of the magnetic character of nanoscale materials, even those embedded in a strongly magnetic host.Keywords
This publication has 20 references indexed in Scilit:
- Irradiation-induced Cu aggregations in Fe: An origin of embrittlement of reactor pressure vessel steelsPhysical Review B, 2001
- Positron confinement in ultrafine embedded particles: Quantum-dot-like state in an Fe-Cu alloyPhysical Review B, 2000
- Understanding Pressure Vessel SteelsMaterials Characterization, 2000
- Anomalous Small-Angle X-Ray Scattering Characterization of Model Pressure Vessel Alloy MicrostructuresMRS Proceedings, 1998
- Increased Elemental Specificity of Positron Annihilation SpectraPhysical Review Letters, 1996
- Microstructural developments in neutron-irradiated mild steel submerged-arc weld metalJournal of Nuclear Materials, 1993
- Microstructural aspects of neutron embrittlement of reactor pressure vessel steels - A view from positron annihilation spectroscopyNuclear Engineering and Design, 1991
- Electron momentum distribution and spin density of ferromagnetic iron studied by spin-polarised positron annihilationJournal of Physics F: Metal Physics, 1988
- Polarized Positron Annihilation in FerromagnetsPhysical Review Letters, 1964
- Polarization of Positrons and Annihilation in Ferromagnetic MaterialsPhysical Review B, 1958