Rational Design of a Flexible CNTs@PDMS Film Patterned by Bio‐Inspired Templates as a Strain Sensor and Supercapacitor

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Abstract
Flexible devices integrated with sensing and energy storage functions are highly desirable due to their potential application in wearable electronics and human motion detection. Here, a flexible film is designed in a facile and low‐cost leaf templating process, comprising wrinkled carbon nanotubes (CNTs) as the conductive layer and patterned polydimethylsiloxane (PDMS) with bio‐inspired microstructure as a soft substrate. Assembled from wrinkled CNTs on patterned PDMS film, a strain sensor is realized to possess sensitive resistance response against various deformations, producing a resistance response of 0.34%, 0.14%, and 9.1% under bending, pressing, and 20% strain, respectively. Besides, the strain sensor can reach a resistance response of 3.01 when stretched to 44%. Furthermore, through the electro‐deposition of polyaniline, the CNTs film is developed into a supercapacitor, which exhibits a specific capacitance of 176 F g−1 at 1 A g−1 and a capacitance retention of 88% after 10 000 cycles. In addition, the fabricated supercapacitor shows super flexibility, delivering a capacitance retention of 98% after 180° bending for 100 cycles, 95% after 45° twisting for 100 cycles, and 98% after 100% stretching for 400 cycles. The superior capacitance stability demonstrates that the design of wrinkled CNTs‐based electrodes fixed by microstructures is beneficial to the excellent electrochemical performance.
Funding Information
  • National Natural Science Foundation of China (51872139, 21501091)
  • Natural Science Foundation of Jiangsu Province (BK20170045)
  • Recruitment Program of Global Experts (1211019)
  • Six Talent Peaks Project in Jiangsu Province (XCL‐043)
  • National Basic Research Program of China (2015CB932200)
  • Nanjing Tech University (3827400203, 50235069)
  • Natural Science Research of Jiangsu Higher Education Institutions of China (18KJB150016)

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