Saturation of Resonant Two-Photon Transitions in Thallium Vapor

Authors:
  • LDL. I. Davis
    L. I. Davis

Abstract
We present direct evidence on the saturation of resonant two-photon transitions in the optical region. Saturation manifests itself as a broadening of the transition linewidth and as a deviation from the low-level intensity dependence for both third-harmonic generation and two-photon-induced fluorescence. These effects may greatly limit the extent of attainable resonant enhancement in experiments which require high intensity for excitation.

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