Expanding the momentum field of view in angle-resolved photoemission systems with hemispherical analyzers
- 1 December 2021
- journal article
- conference paper
- Published by AIP Publishing in Review of Scientific Instruments
- Vol. 92 (12) , 123907
Abstract
In photoelectron spectroscopy, the measured electron momentum range is intrinsically related to the excitation photon energy. Low photon energies eV are commonly encountered in laser-based photoemission and lead to a momentum range that is smaller than the Brillouin zones of most materials. This can become a limiting factor when studying condensed matter with laser-based photoemission. An additional restriction is introduced by widely used hemispherical analyzers that record only electrons photoemitted in a solid angle set by the aperture size at the analyzer entrance. Here, we present an upgrade to increase the effective solid angle that is measured with a hemispherical analyzer. We achieve this by accelerating the photoelectrons toward the analyzer with an electric field that is generated by a bias voltage on the sample. Our experimental geometry is comparable to a parallel plate capacitor, and therefore, we approximate the electric field to be uniform along the photoelectron trajectory. With this assumption, we developed an analytic, parameter-free model that relates the measured angles to the electron momenta in the solid and verify its validity by comparing with experimental results on the charge density wave material TbTe3. By providing a larger field of view in momentum space, our approach using a bias potential considerably expands the flexibility of laser-based photoemission setups.
Keywords
All Related Versions
Funding Information
- U.S. Department of Energy (DE-AC02-76SF00515, DE-AC02-05-CH11231)
- Swiss National Science Foundation (P2EZP2 178542, P2SKP2 184069)
- German Science Foundation (PF 947/1-1)
- Stanford Geballe Laboratory for Advanced Materials Postdoctoral Fellowship Program
This publication has 30 references indexed in Scilit:
- Transient Electronic Structure and Melting of a Charge Density Wave in TbTe 3Science, 2008
- Angle-resolved photoemission study of the evolution of band structure and charge density wave properties in(, La, Ce, Sm, Gd, Tb, and Dy)Physical Review B, 2008
- Development of a momentum microscope for time resolved band structure imagingReview of Scientific Instruments, 2008
- Photoemission momentum mapping and wave function analysis of surface and bulk states on flat Cu(111) and stepped Cu(443) surfaces: A two-photon photoemission studyPhysical Review B, 2008
- Effect of chemical pressure on the charge density wave transition in rare-earth tritelluridesPhysical Review B, 2008
- Energetics and dynamics of unoccupied electronic states at theinterfacePhysical Review B, 2007
- Thermodynamic and transport properties of , , andPhysical Review B, 2006
- Momentum-resolved dynamics of Ar/Cu(1 0 0) interface states probed by time-resolved two-photon photoemissionNew Journal of Physics, 2005
- A very high resolution electron spectrometerJournal of Electron Spectroscopy and Related Phenomena, 1994
- Second-harmonic generation to 2048 Å in Β-Ba2O4IEEE Journal of Quantum Electronics, 1986