This paper reports the successful synthesis of magnetic nanocomposite of calcium ferrite with nitrogen doped graphene oxide (CaFe₂O₄-NGO) for the effective removal of Pb(II) ions and photocatalytic degradation of congo red and p-nitrophenol. X-ray diffraction (XRD), Fourier transform infrared (FT-IR), transmission electron microscopy (TEM), and scanning electron microscopy-energy dispersive X-ray (SEM-EDX) techniques confirmed the presence of NGO and CaFe₂O₄ in the nanocomposite. The Mössbauer studies depicted the presence of paramagnetic doublet and sextet due to presence of CaFe₂O₄ NPs in the nanocomposite. The higher BET surface area in case of CaFe₂O₄-NGO (52.86 m²/g) as compared to CaFe₂O₄ NPs (23.45 m²/g) was ascribed to the effective modulation of surface in the presence of NGO. Adsorption followed the Langmuir model with maximum adsorption capacity of 780.5 mg/g for Pb(II) ions. Photoluminescence spectrum of nanocomposite displayed four-fold decrease in the intensity, as compared to ferrite NPs, thus confirming its high light capturing potential and enhanced photocatalytic activity. The presence of NGO in nanocomposite offered an excellent visible light driven photocatalytic performance. The quenching experiments supported ^●OH and O₂^●− radicals as the main reactive species involved in carrying out the catalytic system. The presence of Pb(II) had synergistic effect on photocatalytic degradation of pollutants. This study highlights the synthesis of CaFe₂O₄-NGO nanocomposite as an efficient adsorbent and photocatalyst for remediating pollutants.

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