RSRajib Sarkar

Rajib Sarkar

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Previous Organizations / Institutes

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Rajib Sarkar has a total of 129 co-authors. Here are the top co-authors by number of shared publications:


Latest Publications

  • Open Access

    NMR evidence of pairing fluctuations above T c and absence of spin magnetism in the time-reversal symmetry-breaking state of Ba 1 − x K x Fe 2 As 2

    by Florian Bärtl, Nadia Stegani, Federico Caglieris, Ilya Shipulin, Yongwei Li, Ruidan Zhong, Quanxin Hu, Yu Zheng, Chi-Ming Yim, Sven Luther, et al.

    Zero-field muon-spin-rotation ( μ SR ) experiments and the observation of a spontaneous Nernst effect indicate broken time-reversal symmetry (BTRS) at T c Z 2 , slightly above the superconducting transition temperature T c in Ba 1 − x K x Fe 2 As 2 , with x ∼ 0.8 . This was interpreted as evidence of a distinct state of matter where BTRS above T c arises from noncondensed Cooper pairs, which maintain long-range interband correlations. However, an inhomogeneous superconducting state competing with magnetism as the origin of the observed behavior cannot be completely ruled out to date. Here, we present detailed As 75 nuclear magnetic resonance (NMR) measurements of Ba 1 − x K x Fe 2 As 2 , with x = 0.766 , yielding T c Z 2 > T c . The NMR data demonstrate that the superconductivity is homogeneous throughout the entire sample volume despite the occurrence of nanoclustering of Ba/K atoms. We observe a suppression of the spin-lattice relaxation rate 1 / T 1 T below the characteristic temperature T * , well above T c . The specific heat yields somewhat lower values of T * , consistent with the microscopic theory of electron quadrupling. The observed monotonous suppression of T * and T c Z 2 in applied magnetic field, the overall temperature dependence of 1 / T 1 T , the NMR spectral characteristics, and the μ SR Knight shift rule out spin magnetism and the proximity to a magnetic instability. We conclude that our data indicate the appearance of pairing fluctuations below T * and that the breaking of time-reversal symmetry represents an unconventional state which is unrelated to spin magnetism.

  • Open Access

    Distinct uniaxial stress and pressure fingerprint of superconductivity in the 3D kagome lattice compound CeRu2

    by O. Gerguri, D. Das, V. Sazgari, H. X. Liu, C. Mielke Iii, P. Král, S. S. Islam, J. N. Graham, V. Grinenko, R. Sarkar, et al.

    The exploration of tunable superconductivity in strongly correlated electron systems is a central pursuit in condensed matter physics, with implications for both fundamental understanding and potential applications. The Laves phase CeRu2, a pyrochlore compound, exhibits a three-dimensional (3D) kagome lattice type geometry giving rise to flat bands and degenerate Dirac points, where band structure features intertwine with strong multi-orbital interaction effects deriving from its correlated electronic structure. Here, we combine muon spin rotation (μSR), uniaxial in-plane stress, and hydrostatic pressure to probe the superconducting state of CeRu2. Uniaxial stress up to 0.22 GPa induces a dome-shaped evolution of the critical temperature Tc, with an initial plateau, successively followed by enhancement and suppression without any structural phase transition. Stress is further found to drive a crossover from anisotropic to isotropic s-wave pairing. In contrast, hydrostatic pressure up to 1.9 GPa leaves Tc largely unchanged but alters the superfluid density from exponential to linear behavior at low temperatures, indicative of nodal superconductivity under hydrostatic pressure. These findings identify CeRu2 as a prime platform for multifold tuning of superconductivity in a 3D correlated material.


  • Open Access

    Contrasting c-axis and in-plane uniaxial stress effects on superconductivity and stripe order in La1.885Ba0.115CuO4

    by Shams Sohel Islam, Vahid Sazgari, Jennifer N. Graham, Orion Gerguri, Petr Král, Ikuya Maetsu, Hrishikesh Gopakumar, Markus Müller, Rajib Sarkar, Vadim Grinenko, et al.

    The cuprate superconductor La2−xBaxCuO4 (LBCO) near x = 0.125 is a striking example of intertwined electronic orders, where 3D superconductivity is anomalously suppressed, allowing spin and charge stripe order to develop. Understanding this interplay remains a key challenge in cuprates, highlighting the necessity of external tuning for deeper insight. While in-plane uniaxial stress enhances superconductivity and suppresses stripe order, the effects of c-axis compression remains largely unexplored. Here, we use muon spin rotation (μSR) and AC susceptibility with an in situ piezoelectric stress device to investigate the spin-stripe order and superconductivity in LBCO-0.115 under c-axis compression. The measurements reveal a gradual suppression of the superconducting transition temperature (Tc) with increasing c-axis stress, in stark contrast to the strong enhancement observed under in-plane stress. We further show that while in-plane stress rapidly reduces both the magnetic volume fraction (Vm) and the spin-stripe ordering temperature (Tso), c-axis compression has no effect, with Vm and Tso exhibiting an almost unchanged behavior up to the highest applied stress of 0.21 GPa. These findings demonstrate a strong anisotropy in stress response.


  • Magnetism in the Kitaev quantum spin liquid candidate RuBr3

    by T. Weinhold, C. Wang, F. Seewald, V. Grinenko, Y. Imai, F. Sato, K. Ohgushi, H.-H. Klauss, R. Sarkar

    The present studies show that long-range magnetic order takes place in RuBr3 at ≈34 K. The observations of clear oscillations in the muon time spectra demonstrate the presence of well-defined internal fields at the muon sites. The magnetic ordering appears to be very robust and static, suggesting a more conventional nature of magnetic ordering in the RuBr3 system at zero field. Present investigations prove that in RuBr3 the Kitaev interactions are likely to be weakened at zero field in comparison to the α−RuCl3 system. This proves that it is possible to tune the Kitaev interactions by replacing Cl with heavier halogen elements such as Br.


  • Open Access

    Magnetism in Kitaev Quantum Spin Liquid Candidate RuBr$_3$

    by T. Weinhold, C. Wang, F. Seewald, V. Grinenko, Y. Imai, F. Sato, K. Ohgushi, H. -H. Klauss, R. Sarkar

    The present studies show that long-range magnetic order takes place in RuBr$_3$ at $\approx$ 34 K. The observations of clear oscillations in the muon time spectra demonstrate the presence of well-defined internal fields at the muon sites. The magnetic ordering appears to be very robust and static suggesting a more conventional nature of magnetic ordering in the RuBr$_3$ system at zero field. Present investigations prove that in RuBr$_3$ the Kitaev interactions are likely to be weakened at zero field in comparison to the $α$-RuCl$_3$ system. This proves that it is possible to tune the Kitaev interactions by replacing Cl with heavier halogen elements such as Br.

  • Open Access

    Static and Resonant Properties and Magnetic Phase Diagram of LiMn2TeO6

    by Tatyana Vasilchikova, Evgeniya Vavilova, Timur Salikhov, Vladimir Nalbandyan, Shanu Dengre, Rajib Sarkar, Hans-Henning Klauss, Alexander Vasiliev

    Physical properties of the mixed-valent tellurate of lithium and manganese, LiMn2TeO6, were investigated in measurements of ac and dc magnetic susceptibility χ, magnetization M, specific heat Cp, electron spin resonance (ESR), and nuclear magnetic resonance (NMR) in the temperature range 2–300 K under magnetic field up to 9 T. The title compound orders magnetically in two steps at T1 = 20 K and T2 = 13 K. The intermediate phase at T2 < T < T1 is fully suppressed by magnetic field µ0H of about 4 T. Besides magnetic phases transitions firmly established in static measurements, relaxation-type phenomena were observed well above magnetic ordering temperature in resonant measurements.


  • Magnetic anisotropy and spin dynamics in the kagome magnet Fe4Si2Sn7O16 : NMR and magnetic susceptibility study on oriented powder

    by S. Dengre, R. Sarkar, L. Opherden, T. Herrmannsdörfer, M. Allison, T. Söhnel, C. D. Ling, J. S. Gardner, H.-H. Klauss

    Fe4Si2Sn7O16 hosts an undistorted kagome lattice of Fe2+ (3d6, S=2) ions. We present results of bulk magnetization and Sn nuclear magnetic resonance (NMR) measurements on an oriented Fe4Si2Sn7O16 powder sample oriented in geometries parallel (∥) and perpendicular (⊥) to the external applied magnetic field used for orienting the powder (Bori). The bulk susceptibility χ shows a broad peak at TN∼3 K associated with antiferromagnetic ordering. NMR spectra indicate the presence of planar anisotropy in the kagome planes. From an analysis of the static NMR shift (K) and dynamic spin-lattice relaxation rate (1/T1) we conclude the presence of dominant magnetic fluctuations in the kagome planes. For the ∥ orientation, K scales linearly with the bulk susceptibility for temperatures down to ∼4 K, while in the ⊥ orientation K starts to deviate strongly below T∼30 K. We associate this deviation with the onset of spin-tilting towards the kagome planes. These correlations are also reflected in the 1/T1 data for the ∥ orientation, which starts to decrease below T∼30 K. In this correlated regime, TN<T< ∼30 K, we discuss the formation of positive chiral spin correlations in the kagome planes.


  • Magnetic field tuning of low-energy spin dynamics in the single-atomic magnet Li2(Li1−xFex)N

    by S. A. Bräuninger, A. Jesche, S. Kamusella, F. Seewald, M. Fix, R. Sarkar, A. A. Zvyagin, H.-H. Klauss

    We present a systematic 57Fe Mössbauer study on highly diluted Fe centers in Li2(Li1−xFex)N single crystals as a function of temperature and magnetic field applied transverse and longitudinal with respect to the single-ion anisotropy axis. Below 30 K, the Fe centers exhibit a giant magnetic hyperfine field of B¯A=70.25(2)T parallel to the axis of strongest electric field gradient V¯zz=−154.0(1)V/Å2. Fluctuations of the magnetic hyperfine field are observed between 50 and 300 K and described by the Blume two-level relaxation model. From the temperature dependence of the fluctuation rate, an Orbach spin-lattice relaxation process is deduced. An Arrhenius analysis yields a single thermal activation barrier of E¯A=570(6)K and an attempt frequency ν¯0=309(10)GHz. Mössbauer spectroscopy studies with applied transverse magnetic fields up to 5 T reveal a large increase of the fluctuation rate by more than one order of magnitude. In longitudinal magnetic fields, a splitting of the fluctuation rate into two branches is observed consistent with a Zeeman induced modification of the energy levels. The experimental observations are qualitatively reproduced by a single-ion effective spin Hamiltonian analysis assuming a Fe1+d7 charge state with the unquenched orbital moment and a J=7/2 ground state. It is demonstrated that a weak axial single-ion anisotropy D of the order of a few Kelvin can cause a two orders of magnitude larger energy barrier for longitudinal spin fluctuations.


  • Impact of disorder on dynamics and ordering in the honeycomb-lattice iridate Na2IrO3

    by R. Sarkar, Z. Mei, A. Ruiz, G. Lopez, H.-H. Klauss, J. G. Analytis, I. Kimchi, N. J. Curro

    Kitaev's honeycomb spin-liquid model and its proposed realization in materials such as α−RuCl3, Li2IrO3, and Na2IrO3 continue to present open questions about how the dynamics of a spin liquid are modified in the presence of non-Kitaev interactions as well as the presence of inhomogeneities. Here we use Na23 nuclear magnetic resonance to probe both static and dynamical magnetic properties in single-crystal Na2IrO3. We find that the NMR shift follows the bulk susceptibility above 30 K but deviates from it below; moreover below TN the spectra show a broad distribution of internal magnetic fields. Both of these results provide evidence for inequivalent magnetic sites at low temperature, suggesting inhomogeneities are important for the magnetism. The spin-lattice relaxation rate is isotropic and diverges at TN, suggesting that the Kitaev cubic axes may control the critical quantum spin fluctuations. In the ordered state, we observe gapless excitations, which may arise from site substitution, emergent defects from milder disorder, or possibly be associated with nearby quantum paramagnetic states distinct from the Kitaev spin liquid.