Steven Dazeley

Water-based liquid scintillator (WbLS) is a hybrid detector medium which has been proposed as a fill material for future large-volume rare event searches, including ν − detectors. This family of scintillating suspensions promises waterlike attenuation and scattering behavior, while offering scintillation light yield for sub-Cherenkov-threshold events. These features may allow for improved vertex and energy resolution, and concomitant improvements in background rejection and particle identification. While subscale measurements of light yield, timing and pulse-shape have been performed in several WbLS formulations, detailed measurements of the attenuation and scattering properties of WbLS remain a critical, unresolved step along the pathway to deployment. In pursuit of a better understanding of these parameters, a “long-arm” attenuation and scattering instrument has been developed at Lawrence Livermore National Laboratory, dubbed LASE (Livermore Attenuation and Scattering Experiment). Optical property measurements have been performed using LASE in DI water, Gd-water, WbLS and Gd-WbLS. Measurements of the optical properties of WbLS (1% LAB-PPO scintillator) provided by Brookhaven National Laboratory demonstrate an attenuation minimum of 4.87 × 10 − 4 ± 1.42 × 10 − 4 cm − 1 at 450 nm, while Gd-loaded WbLS (1% LAB-PPO scintillator, 0.1% Gd) demonstrated a minimum attenuation coefficient of 4.77 × 10 − 4 ± 1.27 × 10 − 4 cm − 1 at the same wavelength. Measurements of scattering in WbLS show a scattering coefficient of 3.39 × 10 − 4 ± 1.98 × 10 − 5 cm − 1 at the 450 nm attenuation minimum, while Gd-WbLS has a scattering coefficient of 2.8 × 10 − 4 ± 1.63 × 10 − 5 cm − 1 at that wavelength. These scattering and attenuation coefficients are significantly larger than measured for DI water at similar wavelengths ( 8.8 × 10 − 5 cm − 1 ± 3.8 × 10 − 5 attenuation at 430 nm, 2.2 × 10 − 5 ± 1.28 × 10 − 6 cm − 1 scattering). Though the WbLS attenuation and scattering coefficients measured are lower than the corresponding values published for ultrapure oils and LAB-PPO liquid scintillator, the material tested attenuates significantly more than water across the blue and green portions of the visible spectrum. This attenuation is markedly stronger at wavelengths under 430 nm.

Antineutrinos are an inextricable element of the fission process. The kiloton-scale KamLAND experiment has demonstrated a capability to detect reactor antineutrinos at a range of a few hundred kilometers. But to detect or rule out the existence of a single small reactor over many kilometers requires a large detector, so large in fact that the optical opacity of the detection medium itself becomes an important factor. If the detector is so large that photons cannot traverse the detector medium to an optical detector, then it becomes impractical. For this reason, gadolinium-doped-water Cherenkov detectors have been proposed for large volumes, due to their appealing light-attenuation properties. Even though Cherenkov emission does not produce many photons and the energy resolution is poor, there may be a place for Gd-doped-water detectors in far-field nuclear-reactor monitoring. In this paper, we focus on the reactor-discovery potential of large-volume Gd-doped-water Cherenkov detectors for nuclear-nonproliferation applications. Realistic background models for the worldwide reactor flux, geoneutrinos, cosmogenic fast neutrons, and detector-associated backgrounds are included. We calculate the detector run time required to detect a small 50-MWt reactor at a variety of stand-off distances as a function of detector size. We highlight that, at present, the photomultiplier-tube dark rate and event reconstruction algorithms are the limiting factors to extending such detectors beyond a fiducial mass of approximately 50 kt.

We present a new analysis of the sensitivity of a water Cherenkov based neutron multiplicity counter for non-destructive assay of trace quantities of 240Pu. The multiplicity counter (Water-based Neutron Detector - WaND) contains 1.0 m3 of water doped with 0.2% gadolinium in the form of a gadolinium salt (0.4% GdCl3). It can be used for testing for the presence of trace quantities of 240Pu within a sample of unknown material by observing the correlated timing behavior of neutron capture candidates in the detector. The new analysis takes advantage of the fact that the detector is comprised almost entirely of a homogeneous medium, which permits the use of a simple model to reproduce the observed neutron capture timing behavior. The results of this analysis indicate that the detector has an absolute neutron detection efficiency of 23.4 ± 1.1%, and is sensitive to a 240Pu mass as small as 2.3 mg (at 1σ) after a 1-hour data acquisition.

We present a measurement of the rate of correlated neutron captures in the WATCHBOY detector, deployed at a depth of approximately 390 meters water equivalent (m.w.e.) in the Kimballton Underground Research Facility (KURF). WATCHBOY consists of a cylindrical 2 ton water target doped with 0.1% gadolinium, surrounded by a 40 ton undoped water hermetic shield. We present a comparison of our results with the expected rate of correlated neutron captures arising from high-energy neutrons incident on the outside of the WATCHBOY shield, predicted by a hybrid fluka-geant4-based simulation. The incident neutron energy distribution used in the simulation was measured by a fast neutron spectrometer, the 1.8 ton Multiplicity and Recoil Spectrometer (MARS) detector, at the same depth. We find that the measured detection rate of two correlated neutrons is consistent with that predicted by simulation. The result lends additional confidence in the detection technique used by MARS, and therefore in the MARS spectra as measured at three different depths. Confirmation of the fast neutron flux and spectrum is important as it helps validate the scaling models used to predict the fast neutron fluxes at different overburdens.

The potential of elastic antineutrino-electron scattering in a Gd-doped water Cherenkov detector to determine the direction of a nuclear reactor antineutrino flux was investigated using the recently proposed WATCHMAN antineutrino experiment as a baseline model. The expected scattering rate was determined assuming a 13-km standoff from a 3.758-GWt light water nuclear reactor and the detector response was modeled using a Geant4-based simulation package. Background was estimated via independent simulations and by scaling published measurements from similar detectors. Background contributions were estimated for solar neutrinos, misidentified reactor-based inverse beta decay interactions, cosmogenic radionuclides, water-borne radon, and gamma rays from the photomultiplier tubes (PMTs), detector walls, and surrounding rock. We show that with the use of low background PMTs and sufficient fiducialization, water-borne radon and cosmogenic radionuclides pose the largest threats to sensitivity. Directional sensitivity was then analyzed as a function of radon contamination, detector depth, and detector size. The results provide a list of experimental conditions that, if satisfied in practice, would enable antineutrino directional reconstruction at 3$\sigma$ significance in large Gd-doped water Cherenkov detectors with greater than 10-km standoff from a nuclear reactor.