Henrik Loos

Interactions between short laser pulses and electron bunches determine a wide range of accelerator applications. Finding spatiotemporal overlap between few-micron-sized optical and electron beams is critical, yet there are few routine diagnostics for this purpose. We present a method for achieving spatiotemporal overlap between a picosecond laser pulse and a relativistic sub-ps electron bunch. The method uses the transient change in optical transmission of a Ce:YAG screen upon irradiation with a short electron bunch to co-time the electron and laser beams. We demonstrate and quantify the performance of this method using an inverse Compton source comprised of a 30 MeV electron beam from an X-band linac focused to a 10 μm spot, overlapped with a joule-class picosecond Yb:YAG laser system. This method is applicable to electron beams with few-microjoule bunch energies and uses standard scintillator screens common in electron accelerators.

Details and design challenges of the photoinjector and interaction point chamber for the Compact X-Ray Light Source (CXLS) at Arizona State University are described. The CXLS uses Inverse Compton Scattering (ICS) to produce X-ray photons with energies in the range of 6-20 keV. The electron beam energy required to produce hard X-rays is reduced since the wavelength of the laser is quite short compared to that of a magnetic undulator. This unique aspect allows the accelerator vault of the CXLS to be much smaller than those in traditional facilities. This extremely compact size leads to much smaller costs and shorter timelines compared to large facilities. We review CXLS design elements and then describe operations experience and equipment upgrades with a focus on the photoinjector laser and the ICS interaction point chamber and their associated controls and beam diagnostics.

A new operating mode has been developed for the Linac Coherent Light Source (LCLS) in which we shape the longitudinal phase space of the electron beam. This mode of operation is realized using a horizontal collimator located in the middle of the first bunch compressor to truncate the head and tail of the beam. With this method, the electron beam longitudinal phase space and current profile are reshaped, and improvement in lasing performance can be realized. We present experimental studies at the LCLS of the beam shaping effects on the free-electron laser performance.

Most experimental studies of cavitation in liquid water at negative pressures reported cavitation at tensions significantly smaller than those expected for homogeneous nucleation, suggesting that achievable tensions are limited by heterogeneous cavitation. We generated tension pulses with nanosecond rise times in water by reflecting cylindrical shock waves, produced by X-ray laser pulses, at the internal surface of drops of water. Depending on the X-ray pulse energy, a range of cavitation phenomena occurred, including the rupture and detachment, or spallation, of thin liquid layers at the surface of the drop. When spallation occurred, we evaluated that negative pressures below −100 MPa were reached in the drops. We model the negative pressures from shock reflection experiments using a nucleation-and-growth model that explains how rapid decompression could outrun heterogeneous cavitation in water, and enable the study of stretched water close to homogeneous cavitation pressures.

Generation of femtosecond to sub-femtosecond pulses is attracting much attention in X-ray free-electron laser user community. One method is to use a slotted, emittance-spoiling foil which was proposed before (P. Emma et al., Phys. Rev. Lett. 92, 074801 (2004)) and has been widely used at the Linac Coherent Light Source. Direct experimental characterization of the slotted-foil performance was previously unfeasible due to a lack of appropriate diagnostics. With a recently installed X-band radio-frequency transverse deflector, we are able to characterize the electron bunch spoiling effect and X-ray pulse when using the slotted foil. We show that few-femtosecond X-ray pulses are generated with flexible control of the single-pulse duration or double-pulse separation with comparison to the theoretical model.

The X-ray free-electron laser has opened a new era for photon science, improving the X-ray brightness by ten orders of magnitude over previously available sources. Similar to an optical laser, the spectral and temporal structure of the radiation pulses can be tailored to the specific needs of many experiments by accurately manipulating the lasing medium, that is, the electron beam. Here we report the generation of mJ-level two-colour hard X-ray pulses of few femtoseconds duration with an XFEL driven by twin electron bunches at the Linac Coherent Light Source. This performance represents an improvement of over an order of magnitude in peak power over state-of-the-art two-colour XFELs. The unprecedented intensity and temporal coherence of this new two-colour X-ray free-electron laser enable an entirely new set of scientific applications, ranging from X-ray pump/X-ray probe experiments to the imaging of complex biological samples with multiple wavelength anomalous dispersion.

Single-cycle terahertz fields generated by coherent transition radiation from a relativistic electron beam are used to study the high field optical response of single crystal GaAs. Large amplitude changes in the sub-band-gap optical absorption are induced and probed dynamically by measuring the absorption of a broad-band optical beam generated by transition radiation from the same electron bunch, providing an absolutely synchronized pump and probe geometry. This modification of the optical properties is consistent with strong-field-induced electroabsorption. These processes are pertinent to a wide range of nonlinear terahertz-driven light-matter interactions anticipated at accelerator-based sources.