Ioan Mihai Pop

We perform nanosecond-resolution multiplexed readout on six same-chip superconducting microwave resonators. This allows us to pinpoint the position of ionizing radiation impacts on the chip by measuring the differential time-of-flight of the generated phonons, inducing correlated errors in the device, thereby implementing an on-chip seismic array. We correlate the phase response of each resonator—a proxy for the absorbed energy—to the distance from the impact point to uncover a millimetric characteristic length for the phonon-mediated radiation poisoning.

A defining characteristic of superconductors is their tendency to expel magnetic fields, yet above a critical threshold, magnetic flux penetrates in discrete quanta carried by Abrikosov vortices ¹ . The superconducting gap is completely suppressed at the vortex core, rendering them dissipative, semi-classical entities that impact applications from high-current-density wires to quantum devices. Material disorder can drive a crossover to vortices that preserve an energy gap at the core ^2–4 , owing to intrinsic ⁵ or emergent granularity on the scale of the coherence length ^2,6 . Although quantum vortex behaviour could emerge in this effective tunnel-junction regime ⁷ , and signatures have been observed in diverse systems ^8–10 , coherent manipulation of vortex states has remained elusive. Here we present evidence that vortices trapped in granular superconducting films can behave as two-level systems, exhibiting microsecond-range quantum coherence and energy relaxation times that reach fractions of a millisecond. Using the tools of circuit quantum electrodynamics ¹¹ , we perform coherent manipulation and quantum non-demolition readout of vortex states in granular aluminium microwave resonators, heralding future directions for quantum information processing, materials characterization and sensing.

Improvements in circuit design and, more recently, in materials and surface cleaning have contributed to a rapid development of coherent superconducting qubits. However, organic resists commonly used for shadow evaporation of Josephson junctions (JJs) pose limitations due to residual contamination, poor thermal stability, and compatibility under typical surface-cleaning conditions. To provide an alternative, we developed an inorganic SiO2/Si3N4 on-chip stencil lithography mask for JJ fabrication. The stencil mask is resilient to aggressive cleaning agents and it withstands high temperatures up to 1200 °C, thereby opening new avenues for JJ material exploration and interface optimization. To validate the concept, we performed shadow evaporation of Al-based transmon qubits followed by stencil mask liftoff using vapor hydrofluoric acid, which selectively etches SiO2. We demonstrate an average T1≈75±11 μs over a 200 MHz frequency range across multiple cooldowns for one device, and T1≈44±8 μs for a second device. These results confirm the compatibility of stencil lithography with state-of-the-art superconducting quantum devices and motivate further investigations into materials engineering, film deposition, and surface cleaning techniques.

Nous avons étudié la dynamique des sauts quantiques de phase (quantum phase-slips) dans différents types de chaînes de jonctions Josephson. Les sauts de phase sont contrôlés par le rapport entre l'énergie Josephson et l'énergie de charge de chaque jonction. Nous avons mesuré l'effet des sauts de phase sur l'état fondamental de la chaîne et nous avons observé l'interférence quantique de sauts de phase (effet Aharonov-Casher). Les résultats de nos mesures sont en très bon accord avec les prédictions théoriques. Nous avons montré qu'une chaîne de jonctions Josephson polarisée en phase, présente un comportement collectif, similaire à un objet macroscopique. Les résultats de cette thèse ouvrent la voie pour la conception de nouveaux circuits Josephson, comme par exemple un qubit topologiquement protégé ou un dispositif quantique pour la conversion courant-fréquence.

For practical superconducting quantum processors, orders of magnitude improvement in coherence is required, motivating efforts to optimize hardware design and explore new materials. Among the latter, the coherence of superconducting transmon qubits has been shown to improve by forming the qubit capacitor pads from α-tantalum, avoiding the metastable β-phase that forms when depositing tantalum at room temperature, and has been previously identified to be a source of microwave losses. In this work, we show lumped element resonators containing β-phase tantalum in the form of inclusions near the metal–substrate interface with internal quality factors (Qi) up to 5.0 ± 2.5×106 in the single photon regime. They perform at least as good as resonators with no sign of the β-phase in x-ray diffraction and thermal quasi-particle loss. Our results indicate that small concentrations of β-phase can be beneficial, enhancing critical magnetic fields and potentially, for improving coherence in tantalum-based superconducting circuits.

A key challenge in achieving scalable fault tolerance in superconducting quantum processors is readout fidelity, which lags behind one- and two-qubit gate fidelity. A major limitation in improving qubit readout is measurement-induced transitions, also referred to as qubit ionization, caused by multiphoton qubit-resonator excitation occurring at specific photon numbers. Since ionization can involve highly excited states, it has been predicted that in transmons—the most widely used superconducting qubit—the photon number at which measurement-induced transitions occur is gate-charge dependent. This dependence is expected to persist deep in the transmon regime where the qubit frequency is gate-charge insensitive. We experimentally confirm this prediction by characterizing measurement-induced transitions with increasing resonator photon population while actively calibrating the transmon’s gate charge. Furthermore, because highly excited states are involved, achieving quantitative agreement between theory and experiment requires accounting for higher-order harmonics in the transmon Hamiltonian.

Superconducting qubits equipped with quantum non-demolition readout and active feedback can be used as information engines to probe and manipulate microscopic degrees of freedom, whether intentionally designed or naturally occurring in their environment. In the case of spin systems, the required magnetic field bias presents a challenge for superconductors and Josephson junctions. Here we demonstrate a granular aluminum nanojunction fluxonium qubit (gralmonium) with spectrum and coherence resilient to fields beyond one Tesla. Sweeping the field reveals a paramagnetic spin-1/2 ensemble, which is the dominant gralmonium loss mechanism when the electron spin resonance matches the qubit. We also observe a suppression of MHz range fast flux noise in magnetic field, suggesting the freezing of surface spins. Using an active state stabilization sequence, the qubit hyperpolarizes long-lived two-level systems (TLSs) in its environment, previously speculated to be spins. Surprisingly, the coupling to these TLSs is unaffected by magnetic fields, leaving the question of their origin open. The robust operation of gralmoniums in Tesla fields offers new opportunities to explore unresolved questions in spin environment dynamics and facilitates hybrid architectures linking superconducting qubits with spin systems.