Christopher David Baird

Bright harmonic radiation from relativistically oscillating laser plasmas offers a direct route for generating extreme electromagnetic fields. Theory predicts that under optimized conditions, the plasma medium can support strong spatiotemporal compression of laser energy in a coherent harmonic focus (CHF), delivering intensity boosts many orders of magnitude greater than the incident driving laser pulse ^1–4 . Although diffraction-limited performance ⁵ (spatial compression) and attosecond phase locking ^6–8 (temporal compression) have been demonstrated experimentally, efficient coupling of relativistically intense laser pulse energy into the emitted harmonic cone has not been realized so far. Here we demonstrate that this highly nonlinear interaction can be tailored to deliver the maximum conversion efficiencies predicted from simulations. By fine-tuning the temporal profile of the driving laser on sub-picosecond (9 mJ between the 12th and 47th harmonics are observed. These results are in agreement with the theoretically expected efficiency dependence on harmonic order, verifying that optimal conditions have been achieved in the generation process. This is the important final element required to achieve the expected intensity boosts from a CHF in experiments. Although obtaining spatiotemporal compression and optimal efficiency simultaneously remains challenging, the path to realizing extreme optical field strengths approaching the critical field of quantum electrodynamics (the Schwinger limit at >10 ^{1 6} V cm ⁻¹ or >10 ²⁹ W cm ⁻² ) is now open, permitting all-optical studies of the quantum vacuum and new frontiers for intense attosecond science.

Betatron x rays generated from laser-wakefield accelerators are a promising source for imaging dynamic processes in materials. Here, we present proof-of-concept imaging of microstructural evolution in a hypermonotectic Al - Bi alloy, which consists of liquid Bi particles in a solid Al matrix. The images capture the elongation and fragmentation of Bi particles upon isothermal annealing. Because of the femtosecond time scale of the betatron source, the images are not subject to motion blur, whereas the accessibility of the source allows for studies of long-term processes such as annealing. The high-resolution data reveal that the evolution of Bi particles is mediated by an interplay of grain-boundary wetting and morphological instability, in stark contrast to an earlier proposal for (inverse) coarsening.

Bright high harmonic radiation from relativistically oscillating laser-plasmas offers a direct route to generating extreme electromagnetic fields. Theory shows that under optimised conditions the plasma medium can support strong spatiotemporal compression of laser energy into a Coherent Harmonic Focus (CHF), delivering intensity boosts many orders of magnitude above that of the incident driving laser pulse. Although diffraction-limited performance (spatial compression) and attosecond phase-locking (temporal compression) have been demonstrated in the laboratory, efficient coupling of highly relativistic laser pulse energy into the emitted harmonic cone has not been realised to date. Here, conclusive evidence confirms that the relativistic laser-plasma interaction can be tailored to deliver the maximum conversion efficiencies predicted from simulations. By fine-tuning the temporal profile of the driving laser pulse on femtosecond timescales, energies > 9 mJ between the 12th and 47th harmonics (18 eV to 73 eV) are observed. These results are shown to be in excellent agreement with the theoretically expected efficiency dependence on harmonic order, indicating that optimal conditions have been achieved in the generation process. This is the important final element required to achieve the expected intensity boosts from a CHF in the laboratory. Although obtaining spatiotemporal compression and optimal efficiency simultaneously remains challenging, the path to realising extreme optical field strengths approaching the critical field of quantum electrodynamics (the Schwinger limit at > 10^16 V/m or > 10^29 W.cm^-2) is now open, permitting all-optical studies of the quantum vacuum and drawing new horizons for intense attosecond science.

We describe a laser–plasma platform for photon–photon collision experiments to measure fundamental quantum electrodynamic processes. As an example we describe using this platform to attempt to observe the linear Breit–Wheeler process. The platform has been developed using the Gemini laser facility at the Rutherford Appleton Laboratory. A laser Wakefield accelerator and a bremsstrahlung convertor are used to generate a collimated beam of photons with energies of hundreds of MeV, that collide with keV x-ray photons generated by a laser heated plasma target. To detect the pairs generated by the photon–photon collisions, a magnetic transport system has been developed which directs the pairs onto scintillation-based and hybrid silicon pixel single particle detectors (SPDs). We present commissioning results from an experimental campaign using this laser–plasma platform for photon–photon physics, demonstrating successful generation of both photon sources, characterisation of the magnetic transport system and calibration of the SPDs, and discuss the feasibility of this platform for the observation of the Breit–Wheeler process. The design of the platform will also serve as the basis for the investigation of strong-field quantum electrodynamic processes such as the nonlinear Breit–Wheeler and the Trident process, or eventually, photon–photon scattering.

We report on the characterisation of an x-ray source, generated by a laser-driven plasma wakefield accelerator. The spectrum of the optimised source was consistent with an on-axis synchrotron spectrum with a critical energy of 13.8 − 1.9 + 2.2 keV and the number of photons per pulse generated above 1 keV was calculated to be 6 − 0.9 + 1.2 × 10 9 . The x-ray beam was used to image a resolution grid placed 37 cm from the source, which gave a measured spatial resolution of 4 µm × 5 µm. The inferred emission region had a radius and length of 0.5 ± 0.2 µm and 3.2 ± 0.9 mm respectively. It was also observed that laser damage to the exit aperture of the gas cell led to a reduction in the accelerated electron beam charge and a corresponding reduction in x-ray flux due to the change in the plasma density profile.

X-ray absorption spectroscopy is a well-accepted diagnostic for experimental studies of warm dense matter. It requires a short-lived X-ray source of sufficiently high emissivity and without characteristic lines in the spectral range of interest. In the present work, we discuss how to choose an optimum material and thickness to get a bright source in the wavelength range 2 Å–6 Å (∼2 keV to 6 keV) by considering relatively low-Z elements. We demonstrate that the highest emissivity of solid aluminum and silicon foil targets irradiated with a 1-ps high-contrast sub-kJ laser pulse is achieved when the target thickness is close to 10 µm. An outer plastic layer can increase the emissivity even further.

A high power laser was used to accelerate electrons in a laser-driven wakefield accelerator. The high energy electrons were then used to generate an x-ray beam by passing them through a converter target. This bremsstrahlung source was characterised and used to perform penetrative imaging of industrially relevant samples. The photon spectrum had a critical energy in excess of 100 MeV and a source size smaller than the resolution of the diagnostic ( ≲ 150 µm). Simulations indicate a significantly smaller source is achievable. Variations in the x-ray source characteristics were realised through changes to the plasma and converter parameters while simulations confirm the adaptability of the source. Imaging of high areal density objects with 150 µm resolution was performed, demonstrating the unique advantages of this novel source.