Durga Bhaktavatsala Rao Dasari

We propose a hybrid quantum system in which a magnet supporting nonreciprocal magnons, chiral magnons, or both mediates the dissipative and unidirectional coupling of spin qubits. By driving the qubits, the steady state of this qubit-qubit coupling scheme becomes the maximally entangled Bell state. We devise a protocol where the system converges to this entangled state and benchmark it including qubit decay and dephasing. The protocol is numerically tested on a hybrid system consisting of nitrogen-vacancy (NV) centers coupled to magnon surface modes of a yttrium iron garnet (YIG) film. We show that the dephasing time of the NV centers forms the bottleneck for achieving the entanglement of NV centers separated by a distance within the magnon coherence length. Our findings identify the key technological requirements and demonstrate a viable route toward steady-state entanglement of solid-state spins over distances of several microns using magnonic quantum networks, expanding the toolbox of magnonics for quantum information purposes.

Quantum token protocols enable unforgeable quantum tokens promising unconditional security beyond classical cryptographic assumptions. We show here that the three stages of the Quantum token protocols involving the preparation, storage, and verification can be made more secure when involving spin-photon interfaces that leverage high-fidelity hybrid tripartite (spin-photon-spin) entanglement, Bell state measurements, and highly coherent spin quantum memories. Further we describe the physical implementation of various stages of the protocol using the hybrid electron and nuclear spins in diamond interfaced with time-bin photons.

Color centers that enable nuclear-spin control without RF fields offer a powerful route towards simplified and scalable quantum devices. Such capabilities are especially valuable for quantum sensing and computing platforms that already find applications in biology, materials science, and geophysics. A key challenge is the coherent manipulation of nearby nuclear spins, which serve as quantum memories and auxiliary qubits but conventionally require additional high-power RF fields which increase the experimental complexity and overall power consumption. Finding systems where both electron and nuclear spins can be controlled using a single MW source is therefore highly desirable. Here, using a modified divacancy center in silicon carbide, we show that coherent control of a coupled nuclear spin is possible without any RF fields. Instead, MW pulses driving the electron spin also manipulate the nuclear spin through hyperfineenhanced effects, activated by a precisely tilted external magnetic field. We demonstrate high-fidelity nuclear-spin control, achieving 89% two-qubit tomography fidelity and nearly T1-limited nuclear coherence times. This approach offers a simplified and scalable route for future quantum applications.

We have recently put forth several schemes of unconventional, nonlinearly-enabled thermodynamic (TD) devices that can operate in either the classical or the quantum domain by transforming thermal-state input in multiple uncorrelated modes into non-gaussian state output in selected modes: a four-mode Kerr-nonlinear interferometer that acts as a heat engine; two coupled Kerr-nonlinear Mach-Zehnder interferometers that act as a phase microscope with unprecedented phase resolution; and a noise sensor that can distinguish between unknown nonlinear quantum processes. These schemes reveal the unique merits of nonlinear TD devices: their ability to act in an autonomous, fully coherent, dissipationless fashion, unlike their conventional counterparts. Here we present the opportunities and challenges facing this new paradigm of nonlinear (NL) quantum and classical TD devices along the following lines: A) Linear versus nonlinear multimode transformations in TD devices: what are the principal distinctions between the two types of transformations? B) Classical versus quantum effects in NL TD devices: what are their main differences? Is quantumness an advantage or a disadvantage? C) Deterministic methods of achieving giant nonlinearity at the few-photon level via coherent processes, including multiatom-bath interactions which can paradoxically yield NL Hamiltonian effects: their comparison with probabilistic, measurement-based methods that can achieve similar NL effects in the quantum domain.

We present a protocol for the ground-state cooling of a tripartite hybrid quantum system, in which a macroscopic oscillator acts as a mediator between a single-probe spin and a remote spin ensemble. In the presence of weak dispersive coupling between the spins and the oscillator, cooling of the oscillator and the ensemble spins can be achieved by exploiting the feedback from frequent measurements of the single-probe spin. We explore the parameter regimes necessary to cool the ensemble, the oscillator, or both to their thermal ground states. This novel cooling protocol shows that, even with only weak dispersive coupling, energy transfer-like effects can be obtained by simply manipulating the probe spin. These results not only contribute to the development of a practical solution for cooling/polarizing large spin ensembles but also provide a relatively simple means of tuning the dynamics of a hybrid system. The proposed protocol thus has broader implications for advancing various quantum technology applications, such as macroscopic quantum state generation and remote sensing.

Charge state instabilities have been a bottleneck for the implementation of solid-state spin systems and pose a major challenge to the development of spin-based quantum technologies. Here we investigate the stabilization of negatively charged nitrogen-vacancy (NV⁻) centers in phosphorus-doped diamond at liquid helium temperatures. Photoionization of phosphorous donors in conjunction with charge diffusion at the nanoscale enhances NV⁰ to NV⁻ conversion and stabilizes the NV⁻ charge state without the need for an additional repump laser. The phosphorus-assisted stabilization is explored and confirmed both with experiments and our theoretical model. Stable photoluminescence-excitation spectra are obtained for NV⁻ centers created during the growth. The fluorescence is continuously recorded under resonant excitation to real-time monitor the charge state and the ionization and recombination rates are extracted from time traces. We find a linear laser power dependence of the recombination rate as opposed to the conventional quadratic dependence, which is attributed to the photo-ionization of phosphorus atoms.

To use batteries as large-scale energy storage systems it is necessary to measure and understand their degradation in-situ and in-operando. As a battery’s degradation is often the result of molecular processes inside the electrolyte, a sensing platform which allows to measure the ions with a high spatial resolution is needed. Primary candidates for such a platform are NV-centers in diamonds. We propose to use a single NV-center to deduce the electric field distribution generated by the ions inside the electrolyte through microwave pulse sequences. We show that the electric field can be reconstructed with great accuracy by using a protocol which includes different variations of the free induction decay to obtain the mean electric field components and a pulse sequence consisting of three polarized π-pulses to measure the electric field’s standard deviation σ E . From a semi-analytical ansatz we find that for a lithium ion battery there is a direct relationship between σ E and the ionic concentration. Our results show that it is therefore possible to use NV-centers as sensors to measure both the electric field distribution and the local ionic concentration inside electrolytes.

Charge state instabilities have been a bottleneck for the implementation of solid-state spin systems and pose a major challenge to the development of spin-based quantum technologies. Here we investigate the stabilization of negatively charged nitrogen-vacancy (NV⁻) centers in phosphorus-doped diamond at liquid helium temperatures. Photoionization of phosphorous donors in conjunction with charge diffusion at the nanoscale enhances NV⁰ to NV⁻ conversion and stabilizes the NV⁻ charge state without the need for an additional repump laser. The phosphorus-assisted stabilization is explored and confirmed both with experiments and our theoretical model. Stable photoluminescence-excitation spectra are obtained for NV⁻ centers created during the growth. The fluorescence is continuously recorded under resonant excitation to real-time monitor the charge state and the ionization and recombination rates are extracted from time traces. We find a linear laser power dependence of the recombination rate as opposed to the conventional quadratic dependence, which is attributed to the photo-ionization of phosphorus atoms.