Shubhayu Chatterjee

The anomalous Hall effect (AHE) in magnetic systems is typically governed by symmetry constraints that require the Hall response to be proportional to the out-of-plane magnetization component. Here we demonstrate the emergence of an unconventional in-plane AHE in a low-dimensional heterostructure. By interfacing a low-symmetry topological semimetal with a ferromagnetic insulator, we realize a system with reduced symmetry in which only a single mirror plane is preserved. When the magnetization acquires a finite component within this mirror plane, the remaining symmetry is broken, enabling a Hall response that depends on both in-plane and out-of-plane magnetization components. Measurements across multiple devices reveal a gate-tunable AHE, indicating electrostatic control of the underlying mechanisms. A minimal symmetry-constrained microscopic model shows that interfacial spin-orbit coupling and exchange interaction are responsible for the observed multidirectional AHE response. Our work establishes a pathway for engineering tunable, symmetry-driven Hall effects in low-dimensional quantum materials.

A central puzzle in strongly correlated electronic phases is strange metallic transport, marked by T-linear resistivity and B-linear magnetoresistance, in sharp contrast with quadratic scalings observed in conventional metals. Here, we demonstrate that proximity to quantum critical points, a recurring motif in the phase diagrams of strange metal candidates, can explain both transport anomalies. We construct and solve a minimal microscopic model by coupling electronic excitations at the Fermi surface to quantum critical bosons via a spatially disordered Yukawa interaction, as well as static pinned domains of density wave order. The resultant transport relaxation rate scales as k_{B}T/ℏ at low magnetic fields, and as an effective Bohr magneton μ[over ˜]_{B}B/ℏ at low temperatures. Further, the magnetoresistance in our model shows a scaling collapse upon rescaling the magnetic field and the resistance by temperature, in agreement with experimental observations.

The nature and spectrum of elementary excitations are defining features of a many-body system. In this study, we used a Rydberg quantum simulator to demonstrate a form of spectroscopy, called quench spectroscopy, that probes these low-energy excitations. We illustrated the method on a two-dimensional simulation of the spin-1/2 dipolar XY model. Through microscopic measurements of the spatial spin correlation dynamics following a quench, we extracted the dispersion relation of the elementary excitations for both ferro- and antiferromagnetic couplings. The ferromagnet exhibits elementary excitations behaving as linear spin waves, whereas in the antiferromagnet, spin waves appear to decay, suggesting the presence of strong nonlinearities. Our demonstration highlights the importance of power-law interactions on the excitation spectrum of a many-body system.

We investigate the spontaneous disintegration of magnons in two-dimensional ferromagnets and antiferromagnets dominated by long-range dipolar interactions. Analyzing kinematic constraints, we show that the unusual dispersion of dipolar ferromagnets in a uniform magnetic field precludes magnon decay at all fields, in sharp contrast to short-range exchange-driven magnets. However, in a staggered magnetic field, magnons can decay in both dipolar ferromagnets and antiferromagnets. Remarkably, such decays do not require a minimum threshold field, and happen over a nearly fixed fraction of the Brillouin zone in the XY limit, highlighting the significant role played by dipolar interactions. In addition, topological transitions in the decay surfaces lead to singularities in the magnon spectrum. Regularizing such singular behavior via a self-consistent approach, we make predictions for dynamical spin correlations accessible to near-term quantum simulators and sensors.

Quantum fluctuations can disrupt long-range order in one-dimensional systems and replace it with the universal paradigm of the Tomonaga-Luttinger liquid (TLL), a critical phase of matter characterized by power-law decaying correlations and linearly dispersing excitations. Using a Rydberg quantum simulator, we study how TLL physics manifests in the low-energy properties of a spin chain, interacting under either the ferromagnetic or the antiferromagnetic dipolar XY Hamiltonian. Following quasiadiabatic preparation, we directly observe the power-law decay of spin-spin correlations in real space, allowing us to extract the Luttinger parameter. In the presence of an impurity, the chain exhibits tunable Friedel oscillations of the local magnetization. Moreover, by utilizing a quantum quench, we directly probe the propagation of correlations, which exhibit a light-cone structure related to the linear sound mode of the underlying TLL. Our measurements demonstrate the influence of the long-range dipolar interactions, renormalizing the parameters of TLL with respect to the case of nearest-neighbor interactions. Finally, comparison to numerical simulations exposes the high sensitivity of TLLs to doping and finite-size effects.

Optical detection of magnetic resonance using quantum spin sensors (QSSs) provides a spatially local and sensitive technique to probe spin dynamics in magnets. However, its utility as a probe of antiferromagnetic resonance (AFMR) remains an open question. We report the experimental demonstration of optically detected AFMR in layered van der Waals antiferromagnets (AFM) up to frequencies of 24 gigahertz. We leverage QSS spin relaxation due to low-frequency magnetic field fluctuations arising from collective dynamics of magnons excited by the uniform AFMR mode. First, through AFMR spectroscopy, we characterize the intrinsic exchange fields and magnetic anisotropies of the AFM. Second, using the localized sensitivity of the QSS, we demonstrate magnon transport over tens of micrometers. Last, we find that optical detection efficiency increases with increasing frequency. This showcases the dual capabilities of QSS as detectors of high-frequency magnetization dynamics and magnon transport, paving the way for understanding and controlling the magnetism of antiferromagnets.

Several strongly correlated metals display B-linear magnetoresistance (LMR) with a universal slope, in sharp contrast to the B 2 scaling predicted by Fermi liquid theory. We provide a unifying explanation of the origin of LMR by focusing on a common feature in their phase diagrams—proximity to symmetry-breaking orders. Specifically, we demonstrate via two microscopic models that LMR with a universal slope arises ubiquitously near ordered phases, provided the order parameter either i) has a finite wave-vector, or ii) has nodes on the Fermi surface. We elucidate the distinct physical mechanisms at play in these two scenarios and derive upper and lower bounds on the field range for which LMR is observed. Finally, we discuss possible extensions of our picture to strange metal physics at higher temperatures and argue that our theory provides an understanding of recent experimental results on thin film cuprates and moiré materials.