Yun-Pil Shim

Typical experimental implementations of single-qubit gates involve two or three fixed rotation axes and up to three rotation steps. In this work, we prove that if the rotation axes can be tuned arbitrarily in a fixed plane, then two rotation steps are sufficient for implementing a single-qubit gate, and one rotation step is sufficient for implementing a state transformation. As concrete examples, we demonstrate two-step single-qubit gate implementations in two different physical qubit systems: (i) a transmon superconducting qubit coupled to an external microwave drive, such as a transmission line; and (ii) a quantum-dot based exchange-only qubit encoded in a three-spin block. These results provide a significant speedup for many common gate implementations, such as Rabi oscillations with phase control.

Monolayer transition metal dichalcogenides host tightly bound excitons, which dominate their optoelectronic response even at room temperatures. Light beams are often used to study these materials with the polarization—often termed the spin angular momentum of the light—providing the mechanism for exciting excitonic states. Light beams, however, can also carry an orbital angular momentum by creating helical structures of their phase front. In this work, we consider a Laguerre-Gaussian beam possessing an orbital angular momentum in addition to the spin angular momentum to create excitons in monolayer transition metal dichalcogenides. We derive optical selection rules that govern the allowed transitions to various exciton series using symmetry arguments. Our symmetry considerations show that we can create dark excitons using these high-order optical beams opening up new avenues for creating long-lived dark excitons with the potential of exploiting them in quantum information processing and storage.

A Pauli spin blockade in quantum dot systems occurs when the charge transport is allowed only for some spin states, and it has been an efficient tool in spin-based qubit devices in semiconductors. We theoretically investigate a Pauli spin blockade in a triple quantum dot molecule consisting of three identical quantum dots in a semiconductor in the presence of an external magnetic field through the molecule. When the three-electron state is on resonance with two- or four-electron states, the Aharonov–Bohm oscillation and the Zeeman splitting lead to a periodic spin blockade effect. We focus on the spin blockade at a two- and three-electron resonance and show that we can tune the magnetic field to selectively allow only either a spin-singlet or spin-triplet state to add an additional electron from tunnel-coupled leads. This spin blockade maintains the three quantum dots at the optimal sweet spot against the charge noise, demonstrating its potential as an efficient readout scheme for the qubits in quantum dot systems.

Resonant transverse driving of a two-level system as viewed in the rotating frame couples two degenerate states at the Rabi frequency, an equivalence that emerges in quantum mechanics. While successful at controlling natural and artificial quantum systems, certain limitations may arise (e.g., the achievable gate speed) due to nonidealities like the counterrotating term. We introduce a superconducting composite qubit (CQB), formed from two capacitively coupled transmon qubits, which features a small avoided crossing—smaller than the environmental temperature—between two energy levels. We control this low-frequency CQB using solely baseband pulses, nonadiabatic transitions, and coherent Landau-Zener interference to achieve fast, high-fidelity, single-qubit operations with Clifford fidelities exceeding 99.7%. We also perform coupled qubit operations between two low-frequency CQBs. This work demonstrates that universal nonadiabatic control of low-frequency qubits is feasible using solely baseband pulses.

We propose a non-destructive means of characterizing a semiconductor wafer via measuring the parameters of an induced quantum dot on the material system of interest with a separate probe chip that can also house the measurement circuitry. We show that a single wire can create the dot, determine if an electron is present, and be used to measure critical device parameters. Adding more wires enables more complicated (potentially multi-dot) systems and measurements. As one application for this concept, we consider a silicon metal-oxide-semiconductor and silicon/silicon-germanium quantum dot qubits relevant to quantum computing and show how to measure low-lying excited states (so-called “valley” states). This approach provides an alternative method for the characterization of parameters that are critical for various semiconductor-based quantum dot devices without fabricating such devices.

We present a theory for understanding the exchange interaction between electron spins in neighboring quantum dots, either by changing the detuning of the two quantum dots or independently tuning the tunneling barrier between quantum dots. The Hubbard model and a more realistic confining-potential model are used to investigate how the tilting and barrier control affect the effective exchange coupling and thus the gate fidelity in both the detuning and symmetric regimes. We show that the exchange coupling is less sensitive to the charge noise through tunnel barrier control (while allowing for exchange coupling operations on a sweet spot where the exchange interaction has zero derivative with respect to the detuning). Both GaAs and Si quantum dots are considered, and we compare our results with experimental data showing qualitative agreements. Our results answer the open question of why barrier gates are preferable to tilt gates for exchange-based gate operations.

We introduce an always-on, exchange-only qubit made up of three localized semiconductor spins that offers a true “sweet spot” to fluctuations of the quantum dot energy levels. Both single- and two-qubit gate operations can be performed using only exchange pulses while maintaining this sweet spot. We show how to interconvert this qubit to other three-spin encoded qubits as a resource for quantum computation and communication.

Superconducting circuits offer tremendous design flexibility in the quantum regime culminating most recently in the demonstration of few qubit systems supposedly approaching the threshold for fault-tolerant quantum information processing. Competition in the solid-state comes from semiconductor qubits, where nature has bestowed some very useful properties which can be utilized for spin qubit-based quantum computing. Here we begin to explore how selective design principles deduced from spin-based systems could be used to advance superconducting qubit science. We take an initial step along this path proposing an encoded qubit approach realizable with state-of-the-art tunable Josephson junction qubits. Our results show that this design philosophy holds promise, enables microwave-free control, and offers a pathway to future qubit designs with new capabilities such as with higher fidelity or, perhaps, operation at higher temperature. The approach is also especially suited to qubits on the basis of variable super-semi junctions.

Recent improvements in materials growth and fabrication techniques may finally allow for superconducting semiconductors to realize their potential. Here, we build on a recent proposal to construct superconducting devices such as wires, Josephson junctions, and qubits inside and out-of single crystal silicon or germanium. Using atomistic fabrication techniques such as STM hydrogen lithography, heavily doped superconducting regions within a single crystal could be constructed. We describe the characteristic parameters of basic superconducting elements-a 1-D wire and a tunneling Josephson junction-and estimate the values for boron-doped silicon. The epitaxial, single-crystal nature of these devices, along with the extreme flexibility in device design down to the single-atom scale, may enable lower noise or new types of devices and physics. We consider applications for such supersilicon devices, showing that the state-of-the-art transmon qubit and the sought-after phase-slip qubit can both be realized. The latter qubit leverages the natural high kinetic inductance of these materials. Building on this, we explore how kinetic inductance-based particle detectors (e.g., photon or phonon) could be realized with potential application in astronomy or nanomechanics. We discuss supersemi devices (such as in silicon, germanium, or diamond) which would not require atomistic fabrication approaches and could be realized today.