Sergey Makarov

Recent research and development into the formation of nanoscale channels as a central component of nanofluidic biochip systems revolutionized the biological and chemical fields. Exploration of new pathways to form nanochannels is increasingly necessary to provide a new generation of analytical tools with accurate control of liquid fluid flow, high selectivity and increased mass flow rate. Here, we demonstrate that a single 9-keV pulse from X-ray free-electron-laser can form a nanoscale mm-long cavity in LiF. The laser-generated shock pressure results in channel formation with >1,000 length-to-diameter aspect ratio. The development of void is analyzed via continuum and atomistic simulations revealing a sequence of processes leading to the final long cavity structure. This work presents the study of mm-long nanochannel formation by a single high-brilliance X-ray free-electron laser pulse. With MHz repetition rate X-ray free electron laser opens a new avenue for the development of lab-on-chip applications in any material, including those non-transparent to optical lasers.

The article deals with the possibility of using high-resolution imaging X-ray spectroscopy to study the parameters of the interaction region of a laser-plasma aluminium supersonic flow (jet) with an argon gas wall in a model experiment with astrophysical similarity to Herbig–Haro objects. Experiments of this kind are promising for the realisation with modern nanosecond laser complexes with a pulse energy of several tens of J up to several kJ (intensity I_las ~ 10¹²–10¹⁴ W/cm²) and can extend the understanding of the processes taking place in the space environment as well as verify existing theoretical models. The modelling of the laboratory object was carried out in 2 stages—first the macroscopic properties of the object were calculated using a hydrodynamic simulation, and then the calculated spatio-temporal profiles of the macroscopic parameters were fed into a non-stationary kinetic code, which was used to model the radiative properties of the process under consideration. It is shown that the simulated X-ray spectrograms allow to estimate the plasma parameters in the interaction region of the laser-plasma jet with the gas cloud based on the relative intensities of the spectral lines of multiply charged argon ions and the location of this region based on the spatial distribution of the argon ion glow.

Optically-transparent LiF film radiation imaging detectors of three different thicknesses, grown by thermal evaporation on Si(100) substrates and irradiated with monochromatic 7 keV X-rays at several doses in the range between 13 and 4.5×10³ Gy, were investigated by fluorescence microscopy to evaluate their visible photoluminescence response of X-ray induced colour centres and their spatial resolution. By edge-enhancement imaging experiments, performed by irradiating LiF film detectors with an Au mesh in front of them, a spatial resolution of ∼0.3 μm was estimated. This high spatial resolution, combined with the large field of view and the wide dynamic range offered by LiF detectors, encourages their use in X-ray imaging and for high-energy density experiments in synchrotron facilities.

The development of diagnostic methods for dense high-temperature plasma exposed to powerful streams of short-wave radiation is of particular relevance in c

Understanding the behavior of matter at extreme pressures of the order of a megabar (Mbar) is essential to gain insight into various physical phenomena at macroscales—the formation of planets, young stars, and the cores of super-Earths, and at microscales—damage to ceramic materials and high-pressure plastic transformation and phase transitions in solids. Under dynamic compression of solids up to Mbar pressures, even a solid with high strength exhibits plastic properties, causing the induced shock wave to split in two: an elastic precursor and a plastic shock wave. This phenomenon is described by theoretical models based on indirect measurements of material response. The advent of x-ray free-electron lasers (XFELs) has made it possible to use their ultrashort pulses for direct observations of the propagation of shock waves in solid materials by the method of phase-contrast radiography. However, there is still a lack of comprehensive data for verification of theoretical models of different solids. Here, we present the results of an experiment in which the evolution of the coupled elastic–plastic wave structure in diamond was directly observed and studied with submicrometer spatial resolution, using the unique capabilities of the x-ray free-electron laser (XFEL). The direct measurements allowed, for the first time, the fitting and validation of the 2D failure model for diamond in the range of several Mbar. Our experimental approach opens new possibilities for the direct verification and construction of equations of state of matter in the ultra-high-stress range, which are relevant to solving a variety of problems in high-energy-density physics.

Here we demonstrate the results of investigating the damage threshold of a LiF crystal after irradiating it with a sequence of coherent femtosecond pulses using the European X-ray Free Electron Laser (EuXFEL). The laser fluxes on the crystal surface varied in the range ∼ 0.015–13 kJ/cm² per pulse when irradiated with a sequence of 1-100 pulses (t_pulse ∼ 20 fs, E_ph = 9 keV). Analysis of the surface of the irradiated crystal using different reading systems allowed the damage areas and the topology of the craters formed to be accurately determined. It was found that the ablation threshold decreases with increasing number of X-ray pulses, while the depth of the formed craters increases non-linearly and reaches several hundred nanometers. The obtained results have been compared with data already available in the literature for nano- and picosecond pulses from lasers in the soft X-ray/VUV and optical ranges. A failure model of lithium fluoride is developed and verified with simulation of material damage under single-pulse irradiation. The obtained damage threshold is in reasonably good agreement with the experimentally measured one.

Passive solid-state detectors based on the visible radiophotoluminescence (RPL) of stable aggregate F₂ and F₃ ⁺ color centers in lithium fluoride (LiF) are successfully used for X-ray imaging and advanced diagnostics of intense X-rays sources. Among their advantages, these detectors offer a wide dynamic range and simplicity of use. They can be read non-destructively using a fluorescence microscope, enabling high spatial resolution over a large field of view. Optically transparent LiF films, of three different increasing thicknesses, were grown by thermal evaporation on glass and silicon substrates and subsequently irradiated with monochromatic 7 keV X-rays at several doses from 1.3 × 10¹ to 4.5 × 10³ Gy at the SOLEIL synchrotron facility. For all the LiF films, the RPL response was found to depend linearly on the irradiation dose, with films grown on Si(100) substrates exhibiting up to a 50% higher response compared to those grown on glass. A minimum dose of 13 Gy was detected, despite the low thickness of the irradiated films. The limited thickness of the homogeneously colored LiF film allowed to obtain a spatial resolution of (0.44 ± 0.04) μm in edge-enhancement imaging experiments conducted by placing an Au mesh in front of the samples.

Possibilities of the Phase-Contrast X-Ray Method in a Laboratory Astrophysical Experiment on the Study of Plasma Instabilities Возможности метода фазово-контрастной рентгенографии в лабораторном астрофизическом эксперименте по изучению плазменных неустойчивостей

In this paper, a computational-theoretical analysis of the possibilities of using the method of phase-contrast X-ray radiography for the study of low-contrast turbulent flows in laser plasma in experiments with astrophysical similarity is carried out. By modeling the passage of hard coherent X-ray radiation through test objects, we studied the parameters of a laboratory experiment that affect the contrast and resolution of the resulting phase-contrast images. The limiting scale for measuring the frequency-spatial spectrum of image power was determined, on which the manifestation of artifacts from the superimposition of diffraction effects from neighboring objects is not yet critical for the correct interpretation of the results. Optimal object-detector distances are found that provide resolution of the power spectrum of a turbulent flow on micron scales. These results are relevant for future laboratory experiments on the development of instabilities in plasma with astrophysical similarity up to the stage of energy dissipation.

The application of fluorescent crystal media in wide-range X-ray detectors provides an opportunity to directly image the spatial distribution of ultra-intense X-ray beams including investigation of the focal spot of free-electron lasers. Here the capabilities of the micro- and nano-focusing X-ray refractive optics available at the High Energy Density instrument of the European XFEL are reported, as measured in situ by means of a LiF fluorescent detector placed into and around the beam caustic. The intensity distribution of the beam focused down to several hundred nanometers was imaged at 9 keV photon energy. A deviation from the parabolic surface in a stack of nanofocusing Be compound refractive lenses (CRLs) was found to affect the resulting intensity distribution within the beam. Comparison of experimental patterns in the far field with patterns calculated for different CRL lens imperfections allowed the overall inhomogeneity in the CRL stack to be estimated. The precise determination of the focal spot size and shape on a sub-micrometer level is essential for a number of high energy density studies requiring either a pin-size backlighting spot or extreme intensities for X-ray heating.