Jiasheng Chen
Current Organizations / Institutes
The organizations/institutes from the scholar's latest article
Research Subjects
Research Interests
Jiasheng Chen has a total of 60 co-authors. Here are the top co-authors by number of shared publications:
- Friedrich Malte Grosche
University of Cambridge
8 shared publications Jacintha Banda
Max Planck Institute for Chemical Physics of Solids, Dresden, Germany
2 shared publications- Keiron Murphy
Cavendish Laboratory, University of Cambridge, Cambridge CB3 0HE, United Kingdom
2 shared publications - Konstantin Semeniuk
Max Planck Institute for Chemical Physics of Solids
2 shared publications Manuel Brando
Max Planck Institute for Chemical Physics of Solids, Dresden, Germany
2 shared publications- Monika Gamża
Jeremiah Horrocks Institute for Mathematics, Physics and Astronomy, University of Central Lancashire, Preston PR1 2HE, United Kingdom
2 shared publications
Latest Publications
- Open Access
- 10 June 2025
- Published by American Physical Society (APS) in Physical Review Letters
- Vol. 134 (23) , 236501
Magnetic Signatures of Pressure-Induced Multicomponent Superconductivity inThe phase diagram of the heavy fermion compound UTe 2 contains multiple superconducting phases, several of which show characteristics of odd-parity pairing. We have investigated the pressure dependence of the superconducting transition in high-quality crystals of UTe 2 by tracking its signature in the magnetic susceptibility χ ( T ) . A single, sharp superconducting transition is observed at low pressures < 0.3 GPa . At higher pressure, a second feature emerges in χ ( T ) , which is located at the lower-temperature superconducting phase boundary previously identified in specific heat measurements. This second transition anomaly in χ ( T ) can be attributed to a step change in the London penetration depth, providing direct evidence for a change in the superconducting order parameter of UTe 2 . Thermodynamic constraints suggest that the low temperature, high pressure superconducting state is distinct from zero pressure superconductivity as well as from the high pressure, high temperature superconducting state, raising the possibility of multicomponent superconductivity in high pressure UTe 2 . Published by the American Physical Society 2025
- 10 June 2025
- Published by American Physical Society (APS) in Physical Review Letters
- Vol. 134 (23) , 236501
Open AccessMagnetic Signatures of Pressure-Induced Multicomponent Superconductivity inThe phase diagram of the heavy fermion compound UTe 2 contains multiple superconducting phases, several of which show characteristics of odd-parity pairing. We have investigated the pressure dependence of the superconducting transition in high-quality crystals of UTe 2 by tracking its signature in the magnetic susceptibility χ ( T ) . A single, sharp superconducting transition is observed at low pressures < 0.3 GPa . At higher pressure, a second feature emerges in χ ( T ) , which is located at the lower-temperature superconducting phase boundary previously identified in specific heat measurements. This second transition anomaly in χ ( T ) can be attributed to a step change in the London penetration depth, providing direct evidence for a change in the superconducting order parameter of UTe 2 . Thermodynamic constraints suggest that the low temperature, high pressure superconducting state is distinct from zero pressure superconductivity as well as from the high pressure, high temperature superconducting state, raising the possibility of multicomponent superconductivity in high pressure UTe 2 . Published by the American Physical Society 2025
- Open Access
- 26 April 2024
- Published by Springer Nature in Communications Materials
- Vol. 5 (1) , 1-7
Metallic local-moment magnetocalorics as a route to cryogenic refrigeration
Commercial adiabatic demagnetisation refrigerators still employ the same hydrated salts that were first introduced over 85 years ago. The inherent limitations of these insulating magnetocalorics – poor thermal conductivity at sub-Kelvin temperatures, low entropy density, corrosiveness – can be overcome by a new generation of rare-earth based metallic magnetocalorics. Here, we present the metallic magnetocaloric YbNi1.6Sn as an attractive alternative to conventional refrigerants. YbNi1.6Sn retains high entropy into the 100 mK regime and avoids the noble metal constituents of alternative refrigerants. Demagnetisation tests demonstrate that YbNi1.6Sn enables economical and durable alternatives to traditional cooling devices for temperatures reaching below 120 mK. We find that the magnetocaloric properties of this material are facilitated by unusually small Kondo and RKKY interactions, which position YbNi1.6Sn in the extreme local moment limit on the generalised Kondo lattice phase diagram.
- 26 April 2024
- Published by Springer Nature in Communications Materials
- Vol. 5 (1) , 1-7
Open AccessMetallic local-moment magnetocalorics as a route to cryogenic refrigeration
Commercial adiabatic demagnetisation refrigerators still employ the same hydrated salts that were first introduced over 85 years ago. The inherent limitations of these insulating magnetocalorics – poor thermal conductivity at sub-Kelvin temperatures, low entropy density, corrosiveness – can be overcome by a new generation of rare-earth based metallic magnetocalorics. Here, we present the metallic magnetocaloric YbNi1.6Sn as an attractive alternative to conventional refrigerants. YbNi1.6Sn retains high entropy into the 100 mK regime and avoids the noble metal constituents of alternative refrigerants. Demagnetisation tests demonstrate that YbNi1.6Sn enables economical and durable alternatives to traditional cooling devices for temperatures reaching below 120 mK. We find that the magnetocaloric properties of this material are facilitated by unusually small Kondo and RKKY interactions, which position YbNi1.6Sn in the extreme local moment limit on the generalised Kondo lattice phase diagram.
- Open Access
- 17 November 2023
- Published by Royal Society of Chemistry (RSC) in Journal of Materials Chemistry A
- Vol. 11 (48) , 26474-26480
Dy(OH) 3 : a paramagnetic magnetocaloric material for hydrogen liquefaction
Dy(OH) 3 has impressive magnetocaloric performance optimised around 20 K making it suitable for hydrogen liquefaction using magnetic cooling.
- 17 November 2023
- Published by Royal Society of Chemistry (RSC) in Journal of Materials Chemistry A
- Vol. 11 (48) , 26474-26480
Open AccessDy(OH) 3 : a paramagnetic magnetocaloric material for hydrogen liquefaction
Dy(OH) 3 has impressive magnetocaloric performance optimised around 20 K making it suitable for hydrogen liquefaction using magnetic cooling.
- Open Access
- 10 July 2023
- Published by American Physical Society (APS) in Physical Review Letters
- Vol. 131 (2) , 026001
Superconductivity beyond the Conventional Pauli Limit in High-PressureWe report the discovery of superconductivity at a pressure-induced magnetic quantum phase transition in the Kondo lattice system , sustained up to magnetic fields that exceed the conventional Pauli limit eightfold. Like , is locally noncentrosymmetric around the Ce site, but the evolution of critical fields and normal state properties as is tuned through the quantum phase transition motivates a fundamentally different explanation for its resilience to applied field.- 10 July 2023
- Published by American Physical Society (APS) in Physical Review Letters
- Vol. 131 (2) , 026001
Open AccessSuperconductivity beyond the Conventional Pauli Limit in High-PressureWe report the discovery of superconductivity at a pressure-induced magnetic quantum phase transition in the Kondo lattice system , sustained up to magnetic fields that exceed the conventional Pauli limit eightfold. Like , is locally noncentrosymmetric around the Ce site, but the evolution of critical fields and normal state properties as is tuned through the quantum phase transition motivates a fundamentally different explanation for its resilience to applied field. - 20 July 2022
- Published by American Physical Society (APS) in Physical Review Letters
- Vol. 129 (4) , 046402
Fermi Surface and Mass Renormalization in the Iron-Based SuperconductorInteraction-enhanced carrier masses are central to the phenomenology of iron-based superconductors. Quantum oscillation measurements in the new unconventional superconductor resolve all four Fermi surface pockets expected from band structure calculations, which predict an electron pocket in the Brillouin zone corner and three hole pockets enveloping the centers of the top and bottom of the Brillouin zone. Carrier masses reach up to 20 times the bare electron mass and are among the highest ever observed in any iron-based material, accounting for the enhanced heat capacity Sommerfeld coefficient . Mass renormalization is uniform across reciprocal space, suggesting predominantly local correlations, as in the Hund’s metal scenario.- 20 July 2022
- Published by American Physical Society (APS) in Physical Review Letters
- Vol. 129 (4) , 046402
Fermi Surface and Mass Renormalization in the Iron-Based SuperconductorInteraction-enhanced carrier masses are central to the phenomenology of iron-based superconductors. Quantum oscillation measurements in the new unconventional superconductor resolve all four Fermi surface pockets expected from band structure calculations, which predict an electron pocket in the Brillouin zone corner and three hole pockets enveloping the centers of the top and bottom of the Brillouin zone. Carrier masses reach up to 20 times the bare electron mass and are among the highest ever observed in any iron-based material, accounting for the enhanced heat capacity Sommerfeld coefficient . Mass renormalization is uniform across reciprocal space, suggesting predominantly local correlations, as in the Hund’s metal scenario.- Open Access
- 13 March 2022
- Published by Elsevier in International Journal of Electrochemical Science
- Vol. 17 (4) , 220440
A beehive-shaped Pd and Ni Nanoparticle Composite Showing Significant Electrocatalytic Activity Towards Ethanol Oxidation Reaction (EOR)
- 13 March 2022
- Published by Elsevier in International Journal of Electrochemical Science
- Vol. 17 (4) , 220440
Open AccessA beehive-shaped Pd and Ni Nanoparticle Composite Showing Significant Electrocatalytic Activity Towards Ethanol Oxidation Reaction (EOR)
- 30 November 2020
- Published by American Physical Society (APS) in Physical Review Letters
- Vol. 125 (23) , 237002
Unconventional Bulk Superconductivity in Single CrystalsSharp superconducting transition anomalies observed in a new generation of single crystals establish that bulk superconductivity is intrinsic to high purity . Low temperature heat capacity measurements suggest a disorder and field dependent residual Sommerfeld coefficient, consistent with disorder-induced in-gap states as expected for a sign-changing order parameter. The sevenfold reduction in disorder scattering in these new crystals to residual resistivities was achieved using a new liquid transport growth technique, paving the way for multiprobe experiments investigating the normal and superconducting states of .- 30 November 2020
- Published by American Physical Society (APS) in Physical Review Letters
- Vol. 125 (23) , 237002
Unconventional Bulk Superconductivity in Single CrystalsSharp superconducting transition anomalies observed in a new generation of single crystals establish that bulk superconductivity is intrinsic to high purity . Low temperature heat capacity measurements suggest a disorder and field dependent residual Sommerfeld coefficient, consistent with disorder-induced in-gap states as expected for a sign-changing order parameter. The sevenfold reduction in disorder scattering in these new crystals to residual resistivities was achieved using a new liquid transport growth technique, paving the way for multiprobe experiments investigating the normal and superconducting states of .- Open Access
- 8 October 2019
- Published by IOP Publishing in Journal of Physics: Materials
- Vol. 3 (1) , 015007
Chemical and structural stability of superconducting In5Bi3 driven by spin–orbit coupling
Relativistic effects play a prominent role in many electronic material properties such as the Rashba and Dresselhaus spin splitting in inversion asymmetric crystals, or the bulk band gap in topological insulators. By contrast, macroscopic material properties are typically not connected to relativistic phenomena. As an exception to this rule, we show that the macroscopic chemical and structural properties of superconducting In5Bi3 are driven by relativistic physics. In the non-relativistic limit In5Bi3 decomposes into elemental indium and bismuth, but the inclusion of relativistic spin–orbit coupling chemically stabilizes the In5Bi3 stoichiometry. Similarly, the structural stability of tetragonal In5Bi3 is driven by the spin–orbit interaction, which eliminates a phonon instability present in the non-relativistic limit. Low-temperature resistivity and heat capacity measurements show that In5Bi3 is a strong coupling superconductor, with a superconducting critical temperature of 4.2 K and a superconducting critical field of 0.3 T. The unconventional interplay between relativity with chemistry and structure, together with the presence of superconductivity, make In5Bi3 a versatile material that provides, for example, a simple model for the study of strong coupling superconductivity in quasiperiodic crystals.
- 8 October 2019
- Published by IOP Publishing in Journal of Physics: Materials
- Vol. 3 (1) , 015007
Open AccessChemical and structural stability of superconducting In5Bi3 driven by spin–orbit coupling
Relativistic effects play a prominent role in many electronic material properties such as the Rashba and Dresselhaus spin splitting in inversion asymmetric crystals, or the bulk band gap in topological insulators. By contrast, macroscopic material properties are typically not connected to relativistic phenomena. As an exception to this rule, we show that the macroscopic chemical and structural properties of superconducting In5Bi3 are driven by relativistic physics. In the non-relativistic limit In5Bi3 decomposes into elemental indium and bismuth, but the inclusion of relativistic spin–orbit coupling chemically stabilizes the In5Bi3 stoichiometry. Similarly, the structural stability of tetragonal In5Bi3 is driven by the spin–orbit interaction, which eliminates a phonon instability present in the non-relativistic limit. Low-temperature resistivity and heat capacity measurements show that In5Bi3 is a strong coupling superconductor, with a superconducting critical temperature of 4.2 K and a superconducting critical field of 0.3 T. The unconventional interplay between relativity with chemistry and structure, together with the presence of superconductivity, make In5Bi3 a versatile material that provides, for example, a simple model for the study of strong coupling superconductivity in quasiperiodic crystals.
- 2 January 2019
- Published by American Physical Society (APS) in Physical Review B
- Vol. 99 (2) , 020501
Composition dependence of bulk superconductivity inIn the layered iron-based superconductor , a high Sommerfeld ratio of and a temperature dependence of the electrical resistivity at low temperature indicate strong electronic correlations and point toward an unconventional pairing state. We have investigated the role of composition and annealing conditions in optimizing the growth of high-quality . Our findings confirm that bulk superconductivity is observed in samples with disorder scattering rates less than . Fe deficiency on the Fe site is identified as the dominant source of disorder, which can be minimized by precipitating from a slightly iron-rich melt, followed by annealing.- 2 January 2019
- Published by American Physical Society (APS) in Physical Review B
- Vol. 99 (2) , 020501
Composition dependence of bulk superconductivity inIn the layered iron-based superconductor , a high Sommerfeld ratio of and a temperature dependence of the electrical resistivity at low temperature indicate strong electronic correlations and point toward an unconventional pairing state. We have investigated the role of composition and annealing conditions in optimizing the growth of high-quality . Our findings confirm that bulk superconductivity is observed in samples with disorder scattering rates less than . Fe deficiency on the Fe site is identified as the dominant source of disorder, which can be minimized by precipitating from a slightly iron-rich melt, followed by annealing.- 22 August 2018
- Published by American Physical Society (APS) in Physical Review Materials
- Vol. 2 (8) , 084409
Quantum critical points in ferroelectric relaxors: Stuffed tungsten bronze and lead pyrochlore ()We have synthesized ceramic specimens of the tetragonal tungsten bronze (KLT) and characterized its phase transition via x-ray diffraction, dielectric permittivity, resonant ultrasonic spectroscopy, and heat capacity measurements. The space group of KLT is reported as both and with the orthorhombic distortion occurring when there are higher partial pressures of volatile K and Li used inside the closed crucibles for the solid state synthesis. The data show strong relaxor behavior, with the temperature at which the two dielectric relative permittivity peaks decreasing, with and as probe frequency is reduced from 1 MHz to 316 Hz. tests show that the data satisfies a Vogel-Fulcher model better than Arrhenius with an extrapolated freezing temperature for and of and and and for (tending to dc). This difference between from real and imaginary values, albeit counterintuitive, is mandatory, according to the theory of Tagantsev. Therefore, by tuning frequency, the transition could be shifted to absolute zero, suggesting KLT has a relaxor-type quantum critical point. In addition, we have reanalyzed the conflicting literature for pyrochlore which suggests that this also has a relaxor-type quantum critical point since the freezing temperature from the Vogel-Fulcher fitting is below absolute zero. Since the transition temperature evidenced in the dielectric data at approximately 100 kHz shifts below 0 K for very low frequencies, this transition would not be seen with heat capacity data collected in the zero-frequency (dc) limit. Both of these materials show promise for possible new relaxor-type quantum critical points with nonperovskite based structures.- 22 August 2018
- Published by American Physical Society (APS) in Physical Review Materials
- Vol. 2 (8) , 084409
Quantum critical points in ferroelectric relaxors: Stuffed tungsten bronze and lead pyrochlore ()We have synthesized ceramic specimens of the tetragonal tungsten bronze (KLT) and characterized its phase transition via x-ray diffraction, dielectric permittivity, resonant ultrasonic spectroscopy, and heat capacity measurements. The space group of KLT is reported as both and with the orthorhombic distortion occurring when there are higher partial pressures of volatile K and Li used inside the closed crucibles for the solid state synthesis. The data show strong relaxor behavior, with the temperature at which the two dielectric relative permittivity peaks decreasing, with and as probe frequency is reduced from 1 MHz to 316 Hz. tests show that the data satisfies a Vogel-Fulcher model better than Arrhenius with an extrapolated freezing temperature for and of and and and for (tending to dc). This difference between from real and imaginary values, albeit counterintuitive, is mandatory, according to the theory of Tagantsev. Therefore, by tuning frequency, the transition could be shifted to absolute zero, suggesting KLT has a relaxor-type quantum critical point. In addition, we have reanalyzed the conflicting literature for pyrochlore which suggests that this also has a relaxor-type quantum critical point since the freezing temperature from the Vogel-Fulcher fitting is below absolute zero. Since the transition temperature evidenced in the dielectric data at approximately 100 kHz shifts below 0 K for very low frequencies, this transition would not be seen with heat capacity data collected in the zero-frequency (dc) limit. Both of these materials show promise for possible new relaxor-type quantum critical points with nonperovskite based structures.