Nathan Jukam

In this study we investigate the electrical properties in the transparent conductive polymer poly(3,4-ethylendioxythiophene):poly(styrene sulfonate) (PEDOT:PSS) and Cu-doped polymer (PEDOT:PSS 1.3% + CuCl₂) using Hall measurements under the Van der Pauw configuration. The influence of doping on the electrical conductivity, Hall mobility, and carrier concentration is demonstrated in Cu-PEDOT:PSS and compared with pure PEDOT:PSS. Through this, we figured out there are difficulties in preparing Cu-doped (PEDOT:PSS 1.3% + CuCl₂) polymeric thin films. The sheet resistance was measured to determine the electrical conductivity, aided by knowledge of the thin film thickness. Temperature dependency was evaluated using a closed cycle cryostat, covering temperatures ranging from 8K to 300 K. These comprehensive measurements provide valuable insights into the electrical behavior and temperature characteristics of PEDOT:PSS and PEDOT:PSS 1.3% + CuCl₂, facilitating the development of high-performance organic electronic devices.

Fano resonances are observed in a composite metamaterial that consists of an electric split ring resonator eSRR and an I-shaped resonator ISR. By adjusting the length of the ISR the degree of asymmetry in the line shape of the composite metamaterial can be controlled and even made to be symmetric. In contrast to other methods to create Fano resonances, the individual modes of the eSRR and ISR have the same symmetry and are not evanescently coupled to each other. The transmission is simulated using the finite difference time domain method and a coupled oscillator model is used to obtain nominal values of the Fano asymmetry factor q. Composite metamaterials and individual eSRR and ISR metamaterials are fabricated, and their transmission is measured with terahertz time-domain spectroscopy.

Two-dimensional spectroscopy is performed on a terahertz (THz) frequency quantum cascade laser (QCL) with two broadband THz pulses. Gain switching is used to amplify the first THz pulse and the second THz pulse is used to probe the system. Fourier transforms are taken with respect to the delay time between the two THz pulses and the sampling time of the THz probe pulse. The two-dimensional spectrum consists of three peaks at (ω_τ = 0, ω_t = ω₀), (ω_τ = ω₀, ω_t = ω₀), and (ω_τ = 2ω₀, ω_t = ω₀) where ω₀ denotes the lasing frequency. The peak at ω_τ = 0 represents the response of the probe to the zero-frequency (rectified) component of the instantaneous intensity and can be used to measure the gain recovery.

Dispersion control is a key objective in the field of photonics and spectroscopy, since it enhances non-linear effects by both enabling phase matching and offering slow light generation. In addition, it is essential for frequency comb generation, which requires a phase-lock mechanism that is provided by broadband compensation of group velocity dispersion (GVD). At optical frequencies, there are several well-established concepts for dispersion control such as prism or grating pairs. However, terahertz dispersion control is still a challenge, thus hindering further progress in the field of terahertz science and technology. In this work, we present a hybrid waveguide with both broadband, tuneable positive and more than octave-spanning negative terahertz GVD on the order of 10⁻²² s²/m, which is suitable for either intra- or extra cavity operation. This new terahertz device will enable ultra-short pulse compression, allow soliton propagation, improve frequency comb operation and foster the development of novel non-linear applications.

The interaction between intersubband resonances (ISRs) and metamaterial microcavities can form a strongly coupled system where new resonances form that depend on the coupling strength. Here we present experimental evidence of strong coupling between the cavity resonance of a THz metamaterial and the ISR in a high electron mobility transistor structure with a triangular confinement. The device is electrically switched from an uncoupled to a strongly coupled regime by tuning the ISR with epitaxially grown transparent gates. An asymmetric triangular potential in the heterostructure enables ultrawide electrical tuning of ISR which is an order of magnitude higher as compared to the equivalent square well. For a single triangular well, we achieve a coupling strength of 0.52 THz, with a normalized coupling ratio of 0.26.

The emission of a quantum cascade laser can be synchronized to the repetition rate of a femtosecond laser through the use of coherent injection seeding. This synchronization defines a sampling coherence between the terahertz laser emission and the femtosecond laser which enables coherent field detection. In this letter the sampling coherence is measured in the time-domain through the use of coherent and incoherent detection. For large seed amplitudes the emission is synchronized, while for small seed amplitudes the emission is non-synchronized. For intermediate seed amplitudes the emission exhibits a partial sampling coherence that is time-dependent.