Benjamin J. Jacot

Recent advances in spintronics suggest that orbital Hall currents generated by charge injection in light metals can provide nonequilibrium angular momentum without relying on strong spin–orbit coupling (SOC). Here, we examine whether such orbital currents can drive domain wall (DW) motion in an amorphous ferrimagnetic alloy, Gd25(Fe9Co1)75 (GFC), where the rare-earth sublattice offers strong SOC for orbital-to-spin conversion. We compare three representative heterostructures: Pt/GFC as a spin Hall reference, light-metal (Mn or Ti)/GFC for direct orbital-current injection, and light-metal/Pt/GFC incorporating an ultrathin Pt layer for orbital-to-spin conversion. Whereas Pt/GFC exhibits robust and reproducible spin–orbit-torque-driven DW motion, no current-driven DW motion is detected in Mn/GFC or Ti/GFC. Second-harmonic Hall measurements nevertheless reveal finite damping-like torques in both Mn/GFC and Ti/GFC, demonstrating that angular-momentum transfer into GFC does occur but is far weaker than in Pt/GFC. Inserting a 1 nm-thick Pt conversion layer strongly enhances the damping-like torque and restores DW motion. Thickness-dependent analysis further shows that DW mobility and depinning thresholds correlate with the interfacial Dzyaloshinskii–Moriya interaction and domain-wall width, highlighting weak torque conversion and insufficient interfacial stabilization of chiral DWs as key challenges for orbital-driven DW motion in light-metal/ferrimagnet heterostructures.

Light is an effective tool to probe the polarization and domain distribution in ferroelectric materials passively, that is, non‐invasively, for example, via optical second harmonic generation (SHG). With the emergence of oxide electronics, there is now a strong demand to expand the role of light toward active control of the polarization. In this work, optical control of the ferroelectric polarization is demonstrated in prototypical epitaxial PbZr_xTi_1−xO₃ (PZT)‐based heterostructures. This is accomplished in three steps, using above‐bandgap UV light, while tracking the response of the polarization with optical SHG. First, it is found that UV‐light exposure induces a transient enhancement or suppression of the ferroelectric polarization in films with an upward‐ or downward‐oriented polarization, respectively. This behavior is attributed to a modified charge screening driven by the separation of photoexcited charge carriers at the Schottky interface of the ferroelectric thin film. Second, by taking advantage of this optical handle on electrostatics, remanent optical poling from a pristine multi‐domain into a single‐domain configuration is accomplished. Third, via thermal annealing or engineered electrostatic boundary conditions, a complete reversibility of the optical poling is further achieved. Hence, this work paves the way for the all‐optical control of the spontaneous polarization in ferroelectric thin films.

Magnetic skyrmions are compact chiral spin textures that exhibit a rich variety of topological phenomena and hold potential for the development of high-density memory devices and novel computing schemes driven by spin currents. Here, we demonstrate the room-temperature interfacial stabilization and current-driven control of skyrmion bubbles in the ferrimagnetic insulator Tm₃Fe₅O₁₂ coupled to Pt, showing the current-induced motion of individual skyrmion bubbles. The ferrimagnetic order of the crystal together with the interplay of spin–orbit torques and pinning determine the skyrmion dynamics in Tm₃Fe₅O₁₂ and result in a strong skyrmion Hall effect characterized by a negative deflection angle and hopping motion. Further, we show that the velocity and depinning threshold of the skyrmion bubbles can be modified by exchange coupling Tm₃Fe₅O₁₂ to an in-plane magnetized Y₃Fe₅O₁₂ layer, which distorts the spin texture of the skyrmions and leads to directional-dependent rectification of their dynamics. This effect, which is equivalent to a magnetic ratchet, is exploited to control the skyrmion flow in a racetrack-like device.