JLJae Hyuck Lee

Jae Hyuck Lee

*This is an algorithmically generated author record based on publicly available information.

Current Organizations / Institutes

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Previous Organizations / Institutes

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Jae Hyuck Lee has a total of 51 co-authors. Here are the top co-authors by number of shared publications:


Latest Publications

  • Competing Ru magnetic orders in the spin-1 X Y pyrochlore Nd 2 Ru 2 O 7

    by Poonam Yadav, Jae Hyuck Lee, Heung-Sik Kim, Dongjoon Song, A. Dominic Fortes, Changyoung Kim, Sungkyun Choi

    Magnetic pyrochlore oxides exhibit various unconventional electronic phases and excitations due to geometric frustration. Recently, a collective magnetic excitation was reported in Raman spectroscopy on a pyrochlore ruthenate ${\mathrm{Nd}}_{2}{\mathrm{Ru}}_{2}{\mathrm{O}}_{7}$. However, its origin remains unclear as the Ru magnetic ground state has been controversial due to sample quality and inconsistent experimental interpretations. Here, we performed neutron diffraction measurements on a high-quality polycrystalline sample with a nearly absent magnetic impurity phase. Magnetic susceptibility and neutron diffraction measurements reveal an intrinsic Ru magnetic transition at around 145.6 K, whereas a controversial magnetic anomaly at around 21 K is suppressed in our sample, indicating that the latter is dominantly from the magnetic impurity phase. Below 145.6 K, well-defined magnetic Bragg peaks from Ru moments were observed, implying well-formed spin-spin correlations. Magnetic refinements combined with magnetic space group analysis revealed competing Ru magnetic structures, supported by density functional theory calculations. Our results suggest that the collective Raman signal may arise from competing Ru magnetic orders. Order-by-disorder and energetic scenarios are discussed as selection mechanisms for the Ru magnetic ground state. This study provides crucial insights into the search for possible order-by-disorder and topological magnetic properties in a less-studied spin-1 pyrochlore.

  • Definitive Fermi-surface mapping of high-purity RuO2 via angle-dependent quantum oscillations

    by Ju Hyeon Kim, Joonyoung Choi, Jae Hyuck Lee, Hoil Kim, Hyeongwoo Seo, Jun Seong Lee, Myeongjun Kang, Eun Sang Choi, Woun Kang, Jong Mok Ok, et al.


  • Open Access

    Anisotropic strain relaxation-induced directional ultrafast carrier dynamics in RuO 2 films

    by Seung Gyo Jeong, In Hyeok Choi, Seungjun Lee, Jin Young Oh, Sreejith Nair, Jae Hyuck Lee, Changyoung Kim, Ambrose Seo, Woo Seok Choi, Tony Low, et al.

    Ultrafast light-matter interactions inspire potential functionalities in picosecond optoelectronic applications. However, achieving directional carrier dynamics in metals remains challenging due to strong carrier scattering within a multiband environment, typically expected for isotropic carrier relaxation. In this study, we demonstrate epitaxial RuO 2 /TiO 2 (110) heterostructures grown by hybrid molecular beam epitaxy to engineer polarization selectivity of ultrafast light-matter interactions via anisotropic strain engineering. Combining spectroscopic ellipsometry, x-ray absorption spectroscopy, and optical pump-probe spectroscopy, we revealed the strong anisotropic transient optoelectronic response at an excitation energy of 1.58 eV in strain-engineered RuO 2 /TiO 2 (110) heterostructures along both in-plane [001] and [1 1 ¯ 0] crystallographic directions. Theoretical analysis identifies strain-induced modifications in band nesting as the underlying mechanism for enhanced anisotropic carrier relaxation observed at this excitation energy. These findings establish epitaxial strain engineering as a powerful tool for tuning anisotropic optoelectronic responses with near-infrared excitations in metallic systems, paving the way for next-generation polarization-sensitive ultrafast optoelectronic devices.


  • Atomically Thin Two-Dimensional Kagome Flat Band on the Silicon Surface

    by Jae Hyuck Lee, Gwan Woo Kim, Inkyung Song, Yejin Kim, Yeonjae Lee, Sung Jong Yoo, Deok-Yong Cho, Jun-Won Rhim, Jongkeun Jung, Gunn Kim, et al.

    In condensed matter physics, the Kagome lattice and its inherent flat bands have attracted considerable attention for their prediction and observation to host a variety of exotic physical phenomena. Despite extensive efforts to fabricate thin films of Kagome materials aimed at modulating flat bands through electrostatic gating or strain manipulation, progress has been limited. Here, we report the observation of a d-orbital hybridized Kagome-derived flat band in Ag/Si(111) 3×3 as revealed by angle-resolved photoemission spectroscopy. Our findings indicate that silver atoms on a silicon substrate form an unconventional distorted breathing Kagome structure, where a delicate balance in the hopping parameters of the in-plane d-orbitals leads to destructive interference, resulting in double flat bands. The exact quantum destructive interference mechanism that forms the flat band is uncovered in a rigorous manner that has not been described before. These results illuminate the potential for integrating metal-semiconductor interfaces on semiconductor surfaces into Kagome physics, particularly in exploring the flat bands of ideal 2D Kagome systems.


  • Linear scaling relationship of Néel temperature and dominant magnons in pyrochlore ruthenates

    by Jae Hyuck Lee, Dirk Wulferding, Junkyoung Kim, Dongjoon Song, Seung Ryong Park, Changyoung Kim

    We present a systematic Raman spectroscopy study on a series of pyrochlore ruthenates, a system which is not yet clearly settled on its magnetic origin and structure. Apart from the Raman-active phonon modes, new peaks that appear in the energy range of 15–35 meV below the Néel temperature (TN) are assigned as one-magnon modes. The temperature evolution of one-magnon modes displays no significant thermal dependence in mode frequencies, while the intensities decrease monotonically. Remarkably, one magnons from all compounds show similar characteristics with a single dominant peak at lower energy and weaker side peaks at a couple of meV higher energy. Most importantly, we uncover a striking proportionality between the dominant magnon mode energies and the TN values. Our results suggest the Ru ions may have similar or the same magnetic phase in all pyrochlore ruthenates of our study. We have thus found an avenue for directly tuning the magnetic exchange interaction by the selection of the A-site ion.


  • Open Access

    Collective magnetic Higgs excitation in a pyrochlore ruthenate

    by Dirk Wulferding, Junkyoung Kim, Mi Kyung Kim, Yang Yang, Jae Hyuck Lee, Dongjoon Song, Dongjin Oh, Heung-Sik Kim, Li Ern Chern, Yong Baek Kim, et al.

    The emergence of scalar Higgs-type amplitude modes in systems where symmetry is spontaneously broken has been a highly successful, paradigmatic description of phase transitions, with implications ranging from high-energy particle physics to low-energy condensed matter systems. Here, we uncover two successive high temperature phase transitions in the pyrochlore magnet Nd2Ru2O7 at TN = 147 K and T* = 97 K, that lead to giant phonon instabilities and culminate in the emergence of a highly coherent excitation. This coherent excitation, distinct from other phonons and from conventional magnetic modes, stabilizes at a low energy of 3 meV. We assign it to a collective Higgs-type amplitude mode, that involves bond energy modulations of the Ru4 tetrahedra. Its striking two-fold symmetry, incompatible with the underlying crystal structure, highlights the possibility of multiple entangled broken symmetries.