Michael Fechner

Chirality is a pervasive property of matter that underpins many important phenomena across physics ¹ , chemistry ² and biology ³ . Given its broad importance, the development of protocols for rational control of chirality in solid-state systems is highly desirable, especially if this effect can be tuned continuously and in two directions. Yet, this goal has remained elusive owing to the absence of a universal conjugate field that couples linearly to this structural order ^4–6 . Here we introduce the piezochiral effect, which enables control of chirality through mechanical strain. We show by symmetry analysis that uniaxial strain induces chirality in a broad class of achiral crystals that host fragments of opposite chirality within each unit cell ^7,8 , an effect that has so far remained unrecognized. The strain-induced handedness can be tuned either by changing the strain direction or by switching between compressive and tensile strain. We experimentally verify this effect in AgGaS ₂ , using measurements of the optical activity under strain. Our discovery establishes a new scheme for chirality control, with potential applications that range from spintronics to asymmetric catalysis, and enantioselective interactions in biosystems.

Cavities provide a means to manipulate the optical and electronic responses of quantum materials by selectively enhancing light-matter interaction at specific frequencies and momenta. While cavities typically involve external structures, exfoliated flakes of van der Waals (vdW) materials can form intrinsic self-cavities due to their small finite dimensions, confining electromagnetic fields into plasmonic cavity modes, characterized by standing-wave current distributions. While cavity-enhanced phenomena are well-studied at optical frequencies, the impact of self-cavities on nonlinear electronic responses—such as directional photocurrent—remains largely unexplored, particularly in the terahertz regime, critical for emerging ultrafast optoelectronic technologies. Here, we report a self-cavity-induced Purcell enhancement of directional photocurrents in the vdW semimetal WTe ₂ . Using ultrafast optoelectronic circuitry, we measured coherent near-field THz emission resulting from nonlinear photocurrents excited at the sample edges. We observed enhanced emission at finite frequencies, tunable via excitation fluence and sample geometry, which we attribute to plasmonic interference effects controlled by the cavity boundaries. We developed an analytical theory that captures the cavity resonance conditions and spectral response across multiple devices. Our findings establish WTe ₂ as a bias-free, geometry-tunable THz emitter and demonstrate the potential of self-cavity engineering for controlling nonlinear, nonequilibrium dynamics in quantum materials.

The exploration of ultrafast phenomena is a frontier of condensed matter research, where the interplay of theory, computation, and experiment is unveiling new opportunities for understanding and engineering quantum materials. With the advent of advanced experimental techniques and computational tools, it has become possible to probe and manipulate nonequilibrium processes at unprecedented temporal and spatial resolutions, providing insights into the dynamical behavior of matter under extreme conditions. These capabilities have the potential to revolutionize fields ranging from optoelectronics and quantum information to catalysis and energy storage. This roadmap captures the collective progress and vision of leading researchers, addressing challenges and opportunities across key areas of ultrafast science and condensed matter. Contributions in this roadmap span the development of ab initio methods for time-resolved spectroscopy, the dynamics of driven correlated systems, the engineering of materials in optical cavities, and the adoption of FAIR principles for data sharing and analysis. Together, these efforts highlight the interdisciplinary nature of ultrafast research and its reliance on cutting-edge methodologies, including quantum electrodynamical density-functional theory, correlated electronic structure methods, nonequilibrium Green’s function approaches, quantum and ab initio simulations.

Ultrafast switching of ferroic phases is an active research area with technological potential. Yet, some key challenges remain, ranging from limited speeds in ferromagnets to intrinsic volatility of switched domains owing to depolarizing fields in ferroelectrics. Unlike these ferroic systems, ferroaxial materials host bistable states that preserve spatial-inversion and time-reversal symmetry and are therefore immune to depolarizing fields but also difficult to manipulate with conventional methods. We demonstrate photo-induced switching of ferroaxial order by engineering an effective axial field composed of circularly driven terahertz phonon modes. A switched ferroaxial domain remains stable for many hours and can be reversed back with a second terahertz pulse of opposite helicity. The effects demonstrated in this work may lead to the development of a robust platform for ultrafast information storage.

Optically enhanced superconductivity in K3C60 is supported by transient optical spectra, by pressure responses, and by ultrafast nonlinear transport measurements. However, the underlying physics and in fact the similarity or dissimilarity to most properties of equilibrium superconductivity are not clear. In this paper, we study the ultrafast voltage response of optically driven K3C60 thin films. Photo-conductive switches are used to measure changes in voltage as a function of time after irradiation, both below and above Tc. These measurements can be understood if one considers the role of granularity in the photo-induced transport response. They reveal fast voltage changes associated with the kinetic inductance of the in-grain carriers and a slower response that may be attributed to Josephson dynamics at the weak links. Fits to the data yield estimates of the in-grain photo-induced superfluid density after the drive and the dynamics of phase slips at the weak links. This work underscores the increasing ability to make electrical measurements at ultrafast speeds in optically driven quantum materials and demonstrates a striking new platform for optoelectronic device applications.

Chirality, a pervasive form of symmetry, is intimately connected to the physical properties of solids, as well as the chemical and biological activity of molecular systems. However, inducing chirality in a nonchiral material is challenging because this requires that all mirrors and all roto-inversions be simultaneously broken. Here, we show that chirality of either handedness can be induced in the nonchiral piezoelectric material boron phosphate (BPO ₄ ) by irradiation with terahertz pulses. Resonant excitation of either one of two orthogonal, degenerate vibrational modes determines the sign of the induced chiral order parameter. The optical activity of the photo-induced phases is comparable to the static value of prototypical chiral α-quartz. Our findings offer new prospects for the control of out-of-equilibrium quantum phenomena in complex materials.

The exploration of ultrafast phenomena is a frontier of condensed matter research, where the interplay of theory, computation, and experiment is unveiling new opportunities for understanding and engineering quantum materials. With the advent of advanced experimental techniques and computational tools, it has become possible to probe and manipulate nonequilibrium processes at unprecedented temporal and spatial resolutions, providing insights into the dynamical behavior of matter under extreme conditions. These capabilities have the potential to revolutionize fields ranging from optoelectronics and quantum information to catalysis and energy storage. This Roadmap captures the collective progress and vision of leading researchers, addressing challenges and opportunities across key areas of ultrafast science. Contributions in this Roadmap span the development of ab initio methods for time-resolved spectroscopy, the dynamics of driven correlated systems, the engineering of materials in optical cavities, and the adoption of FAIR principles for data sharing and analysis. Together, these efforts highlight the interdisciplinary nature of ultrafast research and its reliance on cutting-edge methodologies, including quantum electrodynamical density-functional theory, correlated electronic structure methods, nonequilibrium Green's function approaches, quantum and ab initio simulations.

Periodic laser driving, known as Floquet engineering, is a powerful tool to manipulate the properties of quantum materials. Using circularly polarised light, artificial magnetic fields, called Berry curvature, can be created in the photon-dressed Floquet-Bloch states that form. This mechanism, when applied to 3D Dirac and Weyl systems, is predicted to lead to photon-dressed movement of Weyl nodes which should be detectable in the transport sector. The transport response of such a topological light-matter hybrid, however, remains experimentally unknown. Here, we report on the transport properties of the type-II Weyl semimetal T_d-MoTe₂ illuminated by a femtosecond pulse of circularly polarised light. Using an ultrafast optoelectronic device architecture, we observed injection currents and a helicity-dependent anomalous Hall effect whose scaling with laser field strongly deviate from the perturbative laws of nonlinear optics. We show using Floquet theory that this discovery corresponds to the formation of a magnetic Floquet-Weyl semimetal state. Numerical ab initio simulations support this interpretation, indicating that the light-induced motion of the Weyl nodes contributes substantially to the measured transport signals. This work demonstrates the ability to generate large effective magnetic fields (> 30T) with light, which can be used to manipulate the magnetic and topological properties of a range of quantum materials.

Inhomogeneities crucially influence the properties of quantum materials, yet methods that can measure them remain limited and can access only a fraction of relevant observables. For example, local probes such as scanning tunnelling microscopy have documented that the electronic properties of cuprate superconductors are inhomogeneous over nanometre length scales. However, complementary techniques that can resolve higher-order correlations are needed to elucidate the nature of these inhomogeneities. Furthermore, local tunnelling probes are often effective only far below the critical temperature. Here we develop a two-dimensional terahertz spectroscopy method to measure Josephson plasmon echoes from an interlayer superconducting tunnelling resonance in a near-optimally doped cuprate. The technique allows us to study the multidimensional optical response of the interlayer Josephson coupling in the material and disentangle intrinsic lifetime broadening from extrinsic inhomogeneous broadening for interlayer superconducting tunnelling. We find that inhomogeneous broadening persists up to a substantial fraction of the critical temperature, above which this is overcome by the thermally increased lifetime broadening.