JJJulio Larrea Jiménez

Julio Larrea Jiménez

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Current Organizations / Institutes

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Previous Organizations / Institutes

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Julio Larrea Jiménez has a total of 95 co-authors. Here are the top co-authors by number of shared publications:


Latest Publications

  • Open Access

    Reentrant Landau levels in a Dirac topological insulator

    by C. Kaufmann Ribeiro, J. C. Mutch, Q. Jiang, J. P. Ayres-Sims, K. Rubi, C. A. Mizzi, E. A. Peterson, D. Bulmash, J. Singleton, N. Harrison, et al.

    Pentatellurides have emerged as an ideal platform for exploring topological phase transitions and their electronic properties. Positioned at the boundary between a strong and weak topological insulator phase, their low carrier density and linear dispersion enable a three-dimensional Dirac Hamiltonian description. A complete understanding of these materials remains elusive due to unexplained sample variability. In particular, these materials have been shown to host anomalous magnetoresistance including \(\log (B)\)-periodic signals, non-\(\log (B)\) and non-1/B oscillations, in addition to the conventional 1/B quantum oscillations. Differing interpretations invoke many-body effects and there is currently no unified understanding of these oscillations. Here we report non-1/B oscillations in ZrTe5 down to 700 mK and up to 60 T, with a temperature and magnetic field dependence that violates the Lifshitz–Kosevich framework. We show that nonlinear Landau-level back-bending, arising from the interplay of cyclotron energy and strong spin-orbit coupling in a non-interacting Dirac system, captures all observed regimes and provides a foundation for understanding the electron dynamics of Dirac topological insulators beyond the quantum limit.

  • Open Access

    Emergent topological semimetal from quantum criticality

    by D. M. Kirschbaum, L. Chen, D. A. Zocco, H. Hu, F. Mazza, M. Karlich, M. Lužnik, D. H. Nguyen, J. Larrea Jiménez, A. M. Strydom, et al.

    The electronic topology of a material is generally described by its Bloch states and the associated band structure, and can be altered by electron–electron interactions. In metallic systems, the interactions are usually treated through the concept of quasiparticles. Here we investigate what happens if no well-defined quasiparticles are present and show that a topological semimetal phase can emerge from the material’s quantum critical state. Using the non-centrosymmetric heavy-fermion compound CeRu 4 Sn 6 , which is intrinsically quantum critical, we show that the topological phase exhibits a dome structure as a function of the magnetic field and pressure. To understand these results, we study a Weyl–Kondo semimetal model at a Kondo destruction quantum critical point. Indeed, it exhibits features in the spectral function that can define topological crossings beyond the quasiparticle picture. Our results outline the importance of the interplay of quantum critical fluctuations and symmetry to search for other emergent topological phases.


  • Two lock-in amplifiers based 3 ω technique: A practical guide for thermal conductivity experiments in bulk samples

    by A. Henriques, M. Santoma, S. Wirth, J. Larrea Jiménez, V. Martelli

    The accurate determination of thermal conductivity κ(T) in bulk materials at room temperature and above is crucial for evaluating their compatibility for specific applications. The 3ω technique is an established methodology for studying the thermal conductivity of thin films, becoming particularly suitable in the case of bulk specimens for T ≳ 300 K, where standard stationary techniques require significant corrections for radiative losses. Although this method has been employed in several works, it remains not widely adopted because its implementation demands considerable sophistication, including experiment design, thin film deposition techniques, and choices of the geometry of the current/heat transducer, electronics, and analytical treatment of the signals. Based on a critical review of the technique’s key technical aspects, this work provides practical support for a rapid and user-friendly implementation, from the design phase through to execution and analysis. We release a Python-based graphical user interface that supports a quantitative estimation of the investigated temperature profiles based on the geometrical parameters (width/length) of the deposited transducer (heater/thermometer metal line) before an experiment, guaranteeing an optimal design of the experimental conditions for each given material under scrutiny.

  • Role of native point defects and Hg impurities in the electronic properties of Bi4I4

    by Gustavo H. Cassemiro, C. David Hinostroza, Leandro Rodrigues de Faria, Daniel A. Mayoh, Jie Liu, Maria C. O. Aguiar, Martin R. Lees, Geetha Balakrishnan, J. Larrea Jiménez, Antonio Jefferson da Silva Machado, et al.

    We studied the effects of point defects and Hg impurities in the electronic properties of bismuth iodide $({\mathrm{Bi}}_{4}{\mathrm{I}}_{4})$. Our transport measurements after annealing at different temperatures show that the resistivity of ${\mathrm{Bi}}_{4}{\mathrm{I}}_{4}$ depends on its thermal history, suggesting that the formation of native defects and impurities can shape the temperature dependence of electrical resistivity. Our density functional theory calculations indicate that the bismuth and iodine antisites and the bismuth vacancies are the dominant native point defects. We find that bismuth antisites introduce resonant states in the band edges, while iodine antisites and bismuth vacancies lead to a $n$-type and a $p$-type doping of ${\mathrm{Bi}}_{4}{\mathrm{I}}_{4}$, respectively. The Hg impurities are likely to be found at Bi substitutional sites, giving rise to the $p$-type doping of ${\mathrm{Bi}}_{4}{\mathrm{I}}_{4}$. Overall, our findings indicate that the presence of native point defects and impurities can significantly modify the electronic properties, and, thus, impact the resistivity profile of ${\mathrm{Bi}}_{4}{\mathrm{I}}_{4}$ due to modifications in the amount and type of carriers, and the associated defect (impurity) scattering. Our results suggest possible routes for pursuing fine-tuning of the electronic properties of quasi-one-dimensional quantum materials.


  • Structural investigation of the quasi-one-dimensional topological insulator Bi4I4

    by C. David Hinostroza, Leandro Rodrigues de Faria, Gustavo H. Cassemiro, J. Larrea Jiménez, Antonio Jefferson da Silva Machado, Walber H. Brito, Valentina Martelli

    The bismuth halide Bi4I4 undergoes a structural transition around TP∼300K, which separates a high-temperature β phase (T>TP) from a low-temperature α phase (T<TP). α and β phases are suggested to host electronic band structures with distinct topological classifications. Rapid quenching was reported to stabilize a metastable β−Bi4I4 at T<TP, making possible a comparative study of the physical properties of the two phases in the same low-temperature range. In this work, we present a structural investigation of Bi4I4 before and after quenching together with electrical resistivity measurements. We found that rapid cooling does not consistently lead to a metastable β−Bi4I4, and a quick transition to α−Bi4I4 is observed. As a result, the comparison of putative signatures of different topologies attributed to a specific structural phase should be carefully considered. The observed phase instability is accompanied by an increase in iodine vacancies and by a change in the temperature dependence of electrical resistivity, pointing to native defects as a possible origin of our finding. Density functional theory (DFT) calculations support the scenario that iodine vacancies, together with bismuth antisites and interstitials are among the defects that are more likely to occur in Bi4I4 during the growth.


  • Inelastic neutron scattering investigation of the crystal field excitations of NdCo5

    by F. de Almeida Passos, G. J. Nilsen, C. E. Patrick, M. D. Le, G. Balakrishnan, Santosh Kumar, A. Thamizhavel, D. R. Cornejo, J. Larrea Jiménez

    We present an inelastic neutron scattering study of the crystal electric field (CEF) levels in the intermetallic ferrimagnets RECo5 (RE=Nd and Y). In NdCo5, measurements at 5K reveal two levels at approximately 28.9 and 52.9 meV. Crystal-field calculations including the exchange field Bexc from the Co sites account for both of these, as well as the spectrum at temperatures above the spin-reorientation transition at ∼280 K. In particular, it is found that both a large hexagonal crystal field parameter A66〈r6〉 and Bexc are required to reproduce the data, with the latter having a much larger value than that deduced from previous computational and experimental studies. Our study sheds light on the delicate interplay of terms in the rare-earth Hamiltonian of RECo5 systems, and is therefore expected to stimulate further experimental and computational work on the broader family of rare-earth permanent magnets.


  • Thermal diffusivity and its lower bound in orthorhombic SnSe

    by Valentina Martelli, Fabio Abud, Julio Larrea Jiménez, Elisa Baggio-Saitovich, Li-Dong Zhao, Kamran Behnia

    The orthorhombic monochalcogenide SnSe has attracted much attention in recent years as a promising high-temperature thermoelectric material. We present a study of its thermal conductivity and specific heat of SnSe between 2 K and 300 K and quantify its anisotropic thermal diffusivity D. For both crystallographic orientations, thermal diffusivity remains above the recently identified Planckian limit (D>vs2τP, where vs is the sound velocity and τP=ℏ/kBT) and its anisotropy in D is set by the anisotropy of vs. Comparison with cubic members of the IV-VI family leads to a consistent picture, where the diffusivity in all members of the family is set by the product of vs, τP and the ‘melting’ velocity derived from the melting temperature.


  • Top Cited Papers
    Open Access

    A quantum magnetic analogue to the critical point of water

    by J. Larrea Jiménez, S. P. G. Crone, E. Fogh, M. E. Zayed, R. Lortz, E. Pomjakushina, K. Conder, A. M. Läuchli, L. Weber, S. Wessel, et al.

    At the liquid–gas phase transition in water, the density has a discontinuity at atmospheric pressure; however, the line of these first-order transitions defined by increasing the applied pressure terminates at the critical point1, a concept ubiquitous in statistical thermodynamics2. In correlated quantum materials, it was predicted3 and then confirmed experimentally4,5 that a critical point terminates the line of Mott metal–insulator transitions, which are also first-order with a discontinuous charge carrier density. In quantum spin systems, continuous quantum phase transitions6 have been controlled by pressure7,8, applied magnetic field9,10 and disorder11, but discontinuous quantum phase transitions have received less attention. The geometrically frustrated quantum antiferromagnet SrCu2(BO3)2 constitutes a near-exact realization of the paradigmatic Shastry–Sutherland model12,13,14 and displays exotic phenomena including magnetization plateaus15, low-lying bound-state excitations16, anomalous thermodynamics17 and discontinuous quantum phase transitions18,19. Here we control both the pressure and the magnetic field applied to SrCu2(BO3)2 to provide evidence of critical-point physics in a pure spin system. We use high-precision specific-heat measurements to demonstrate that, as in water, the pressure–temperature phase diagram has a first-order transition line that separates phases with different local magnetic energy densities, and that terminates at an Ising critical point. We provide a quantitative explanation of our data using recently developed finite-temperature tensor-network methods17,20,21,22. These results further our understanding of first-order quantum phase transitions in quantum magnetism, with potential applications in materials where anisotropic spin interactions produce the topological properties23,24 that are useful for spintronic applications.


  • Open Access

    Anisotropic Thermopower of the Kondo Insulator $\hbox {CeRu}_4\hbox {Sn}_6$ CeRu 4 Sn 6

    by J. Hänel, H. Winkler, M. Ikeda, J. Larrea J., V. Martelli, A. Prokofiev, E. Bauer, S. Paschen