Lukas Lackner

Structured optical cavities have advanced as a powerful test bed to study lattice Hamiltonians in general, and topological phenomena in particular. The tuning of topological modes, enabled via substantial modifications of emulated lattice potentials, has remained out of experimental reach due to the commonly utilized monolithic cavity samples. Here, we study the Su-Schrieffer-Heeger (SSH) lattice Hamiltonian, which we emulate in a widely tunable open optical cavity strongly coupled to excitons in an integrated WS 2 monolayer. The potential landscape comprises a topological domain boundary hosting a topological, exponentially localized mode at the interface between two lattices characterized by different Zak phases. The mode is spectrally tunable over 80 meV. Moreover, we use the unique tilt tunability of our implementation to transform the SSH lattice into a Stark ladder. This transformation couples the topologically protected defect mode to propagating lattice modes and effectively changes the symmetry of the system. Furthermore, it allows us to directly quantify the Zak-phase difference Δ Z a k = ( 1.07 ± 0.11 ) π between the two topological phases. Our Letter constitutes an important step toward tuning topological lattices to control and guide light on nonlinear chips.

MoTe 2 monolayers and bilayers are unique within the family of van der Waals materials since they pave the way toward atomically thin infrared light-matter quantum interfaces, potentially reaching the important telecommunication windows. Here, we report emergent exciton polaritons based on MoTe 2 monolayers and bilayers in a low-temperature open microcavity in a joint experiment-theory study. Our experiments clearly evidence both the enhanced oscillator strength and enhanced luminescence of MoTe 2 bilayers, signified by a 38% increase of the Rabi splitting and a strongly enhanced relaxation of polaritons to low-energy states. The latter is distinct from polaritons in MoTe 2 monolayers, which feature a bottlenecklike relaxation inhibition. Both the polaritonic spin valley locking in monolayers and the spin-layer locking in bilayers are revealed via the Zeeman effect, which we map and control via the light-matter composition of our polaritonic resonances.

Solid-state single-photon sources are central building blocks in quantum information processing. Atomically thin crystals have emerged as sources of nonclassical light; however, they perform below the state-of-the-art devices based on volume crystals. Here, we implement a bright single-photon source based on an atomically thin sheet of WSe₂ coupled to a tunable optical cavity in a liquid-helium-free cryostat without the further need for active stabilization. Its performance is characterized by high single-photon purity (g⁽²⁾(0) = 4.7 ± 0.7%) and record-high, first-lens brightness of linearly polarized photons of 65 ± 4%, representing a decisive step toward real-world quantum applications. The high performance of our devices allows us to observe two-photon interference in a Hong-Ou-Mandel experiment with 2% visibility limited by the emitter coherence time and setup resolution. Our results thus demonstrate that the combination of the unique properties of two-dimensional materials and versatile open cavities emerges as an inspiring avenue for novel quantum optoelectronic devices.

Engineering non-linear hybrid light-matter states in tailored lattices is a central research strategy for the simulation of complex Hamiltonians. Excitons in atomically thin crystals are an ideal active medium for such purposes, since they couple strongly with light and bear the potential to harness giant non-linearities and interactions while presenting a simple sample-processing and room temperature operability. We demonstrate lattice polaritons, based on an open, high-quality optical cavity, with an imprinted photonic lattice strongly coupled to excitons in a WS₂ monolayer. We experimentally observe the emergence of the canonical band-structure of particles in a one-dimensional lattice at room temperature, and demonstrate frequency reconfigurability over a spectral window exceeding 85 meV, as well as the systematic variation of the nearest-neighbour coupling, reflected by a tunability in the bandwidth of the p-band polaritons by 7 meV. The technology presented in this work is a critical demonstration towards reconfigurable photonic emulators operated with non-linear photonic fluids, offering a simple experimental implementation and working at ambient conditions.