Ian Cox

In an experiment performed at the Facility for Rare Isotope Beams (FRIB) using the FRIB Decay Station initiator, 15 new half-lives of isotopes near ^{54}Ca were measured. A new method of extracting lifetimes from experimental data, taking into account the unknown β-delayed neutron emission branches of very neutron-rich nuclei, was developed to enable systematic uncertainty analysis. The experiment observed a dramatic change in the half-life systematics for the isotopes with neutron number N=34. Beyond N=34, the decline of nuclear lifetime is much slower, leading to longer than anticipated lifetimes for near-dripline nuclei. State-of-the-art shell-model calculations can explain the experimental results, revealing the imprint of shell effects and the need for modification of single-particle neutron states. The results from a newly developed quasirandom-phase approximation model with potential for making global predictions were also tested against the experimental results and good agreement was found.

Alpha particle radioactivity is one of the most striking evidence for the existence of cluster structures in atomic nuclei. During the decay process, a preexisting α particle tunnels through the potential barrier formed by the residual nucleus [1,2]. The degree of preformation of the α particle, a strongly bound system of two protons and two neutrons, is extracted from the data by dividing the α-decay probability by the barrier penetrability for a given particle energy. The preformation probability changes rapidly near nuclear shell closures, which is direct evidence that clustering is connected to nuclear structure [3]. Enhanced preformation was observed in the lightest α-particle emitters, spherical tellurium and xenon isotopes decaying to magic isotopes of tin. Here, we show the most extreme case of α-particle preformation from the measurement of the decay of tellurium-104. With a half-life of 7.2 ^+2.3 _-1.5 nanoseconds, tellurium-104 is the fastest ground state α-emitting nucleus known to date. The deduced preformation demonstrates that the enhancement is greater for tellurium-104 than for any other nucleus. One nuclear model that can explain our observation postulates that the α particle can exist only in the low nuclear matter density regions on the surface of the nucleus. The uniquely high preformation for tellurium-104 is attributed to its relation to doubly-magic tin-100, creating conditions conducive to form an α particle.

The 247-keV state in ^{54}Sc, populated in the β decay of ^{54}Ca, is reported here as a nanosecond isomer with a half-life of 26.0(22) ns. The state is interpreted as the 1^{+} member of the πf_{7/2}⊗νf_{5/2} spin-coupled multiplet, which decays to the 3^{+},πf_{7/2}⊗νp_{1/2} ground state. The new half-life corresponds to a pure E2 transition with a strength of 1.93(16) W.u., providing the most precise, unambiguous B(E2) value in the neutron-rich fp region to date for a nucleus with valence protons above Z=20. Notably, it is roughly 4 times larger than the B(E2;1/2^{-}→5/2^{-}) value in ^{55}Ca. The results, as compared to semiempirical and ab initio shell-model calculations, indicate (1) a weak N=34 subshell gap relative to N=32, (2) a large E2 enhancement in Sc as compared to Ca due to 1p-1h proton excitations across Z=28, and (3) empirical effective proton and neutron charges e_{π}=1.30(8)e and e_{ν}=0.452(7)e, respectively, that are in contrast to reports of e_{π}≈1.1-1.15e and e_{ν}≈0.6-0.8e for fp-shell nuclei near N=Z. We demonstrate that these reports are erroneous and that, in fact, a universal set of effective charges can be used across the sd and fp shells.