Yating Zhang

Cloud-aerosol interactions represent a critical uncertainty in climate systems. Using 2006–2021 CALIPSO products, we investigated upper tropospheric clouds and aerosol layers across four Russian regions: Western Plains, West Siberian Plain, Central Siberian Plateau, and Eastern Mountains. Top Cloud Optical Depth (TCOD), Top Depolarization Ratio of clouds (TDRc), and Layer Level (LLc) exhibit pronounced seasonal and diurnal variations, peaking during summer and nighttime when convection intensifies. Upper aerosol layers show low Total Aerosol Optical Depth (TAOD) and Color Ratio (CRa), often displaying multi-layered structures influenced by spring–summer dust transport and biomass burning. We constructed a correlation matrix of 49 parameter pairs (7 cloud × 7 aerosol parameters), revealing moderate positive correlations between cloud and aerosol layer heights under coexistence conditions. TDRc showed weak linear but strong nonlinear relationships with aerosol parameters, indicating complex coupling mechanisms beyond simple linear models. Nighttime observations demonstrated superior signal-to-noise ratios and correlation coefficients compared to daytime measurements. These findings enhance understanding of cloud-aerosol coupling at middle-high latitudes, providing parameterization constraints for improving global climate model representations of these processes.

This study utilized Cloud–Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) satellite level-2 data with high-confidence cloud–aerosol discrimination (|CAD| > 70) to investigate the optical properties, vertical distributions, seasonal variations, and aerosol interactions of near-surface cloud layers (cloud base height < 2.5 km) over Australia from 2006 to 2021. This definition encompasses both traditional low clouds and part of mid-level clouds that extend into the lower troposphere, enabling a comprehensive view of cloud systems that interact most directly with boundary-layer aerosols. The results showed that the optical depth of low clouds (CODL) exhibited significant spatial heterogeneity, with higher values in central and eastern regions (often exceeding 6.0) and lower values in western plateau regions (typically 4.0–5.0). CODL values demonstrated clear seasonal patterns with spring peaks across all regions, contrasting with traditional summer-maximum expectations. Pronounced diurnal variations were observed, with nighttime CODL showing systematic enhancement effects (up to 19.29 maximum values compared to daytime 11.43), primarily attributed to surface radiative cooling processes. Cloud base heights (CBL) exhibited counterintuitive nighttime increases (41% on average), reflecting fundamental differences in cloud formation mechanisms between day and night. The geometric thickness of low clouds (CTL) showed significant diurnal contrasts, decreasing by nearly 50% at night due to enhanced atmospheric stability. Cloud layer number (CN) displayed systematic nighttime reductions (18% decrease), indicating dominance of single stratiform cloud systems during nighttime. Regional analysis revealed that the central plains consistently exhibited higher CODL values, while eastern mountains showed elevated cloud heights due to orographic effects. Correlation analysis between cloud and aerosol layer properties revealed moderate but statistically significant relationships (|R| = 0.4–0.6), with the strongest correlations appearing between cloud layer heights and aerosol layer heights. However, these correlations represent only partial influences among multiple factors controlling cloud development, suggesting measurable but modest aerosol effects on cloud properties. This study provides comprehensive observational evidence for cloud optical property variations and aerosol–cloud interactions over Australia, contributing to an improved understanding of Southern Hemisphere cloud systems and their climatic implications.