Observation of Two Nondispersive Magnetic Excitations in NiO by Resonant Inelastic Soft-X-Ray Scattering

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Abstract
We present high resolution (ΔE=120  meV) resonant inelastic x-ray scattering data measured at the Ni L3 edge (2p3/2→3d) on the paradigmatic antiferromagnetic oxide NiO. Spectra reveal clear signatures of magnetic excitations at ∼95 and ∼190  meV whose energy seems independent from transferred momentum. These spectral features are well reproduced by a single Ni2+ ion model in an effective exchange field. Within this local model the two magnetic excitations are characterized by a variation of the atomic magnetic moment along the local ordering direction (ΔSα) of one and two units. The ΔSα=2 case has different nature from bimagnons observed in optical Raman spectra, for which ΔSα=0.

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