Tyler James Quill
Current Organizations / Institutes
The organizations/institutes from the scholar's latest article
Research Subjects
Research Interests
Tyler James Quill has a total of 16 co-authors. Here are the top co-authors by number of shared publications:
- Adam Marks
Stanford University
1 shared publication - Alberto Salleo
Department of Materials Science and Engineering, Stanford University, Stanford, USA
1 shared publication - Arianna Magni
Stanford University
1 shared publication - Arwin Goossens
Hasselt University
1 shared publication - Christina Cheng
Stanford University
1 shared publication - Garrett Lecroy
Stanford University
1 shared publication
Latest Publications
- Open Access
- 4 September 2025
- Published by American Chemical Society (ACS) in ChemRxiv
Revealing the Full Potential of Mixed Ionic-Electronic Semiconductors – Avoiding Homocoupling to Boost Electrochemical Transistor Performance
Organic electrochemical transistors (OECTs) enable the transduction of ionic signals into electronic outputs, positioning them as ideal candidates for next-generation sensing and (bio)signal processing applications. Recent years have witnessed the development of various OECT channel materials, affording insights on structural fine-tuning to achieve optimal performance and/or stability. However, homocouplings, commonly present in alternating conjugated polymers, have largely been overlooked. This study investigates the effect of homocoupling on OECT materials by employing two synthesis methods – standard Stille polymerization and an alternative symmetric approach – to create the p-type enhancement-mode benchmark polymer pgBTTT. The impact of homocoupling, and its absence, is studied by comparing the bulk properties of the two polymers and evaluating their respective OECT metrics. The new, homocoupling-free polymer exhibits a notably improved OECT performance (μC*), mainly due to an increase in electronic mobility (μ), which is attributed to both the perfectly alternating structure and its higher molar mass.
- 4 September 2025
- Published by American Chemical Society (ACS) in ChemRxiv
Open AccessRevealing the Full Potential of Mixed Ionic-Electronic Semiconductors – Avoiding Homocoupling to Boost Electrochemical Transistor Performance
Organic electrochemical transistors (OECTs) enable the transduction of ionic signals into electronic outputs, positioning them as ideal candidates for next-generation sensing and (bio)signal processing applications. Recent years have witnessed the development of various OECT channel materials, affording insights on structural fine-tuning to achieve optimal performance and/or stability. However, homocouplings, commonly present in alternating conjugated polymers, have largely been overlooked. This study investigates the effect of homocoupling on OECT materials by employing two synthesis methods – standard Stille polymerization and an alternative symmetric approach – to create the p-type enhancement-mode benchmark polymer pgBTTT. The impact of homocoupling, and its absence, is studied by comparing the bulk properties of the two polymers and evaluating their respective OECT metrics. The new, homocoupling-free polymer exhibits a notably improved OECT performance (μC*), mainly due to an increase in electronic mobility (μ), which is attributed to both the perfectly alternating structure and its higher molar mass.